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Towards the Synthesis of Atomic Scale Wires

  • P. A. Anderson (a1), L. J. Woodall (a1), A. Porch (a2), A. R. Armstrong (a1), I. Hussain (a1) and P. P. Edwards (a1)...

Abstract

Recent work1 has highlighted the possibility that through the introduction of metals into the one-dimensional channels of zeolite L, it may be feasible to engineer charge transport along the channels to produce a unique compound comprising a precise, assembled array of ultrafine, atomic-scale conducting wires embedded within the aluminosilicate framework. Using electron spin resonance (ESR), and microwave cavity perturbation measurements, we examine the properties of these remarkable materials as a function of composition as they approach the insulator to metal transition.

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1. Anderson, P. A., Armstrong, A. R., Edwards, P. P., Angew. Chem. 106, 669 (1994); Angew. Chem., Int. Ed. Engl. 33, 641 (1994).
2. Rabo, J. A., Angell, C. L., Kasai, P. H., Schomaker, V., Discuss. Faraday Soc. 41, 328 (1966).
3. Edwards, P. P., Harrison, M. R., Klinowski, J., Ramdas, S., Thomas, J. M., Johnson, D. C., Page, C. J., J. Chem. Soc., Chem. Commun., 982 (1984).
4. Harrison, M. R., Edwards, P. P., Klinowski, J., Thomas, J. M., Johnson, D. C., Page, C. J., J. Solid State Chem. 54, 330 (1984).
5. Anderson, P. A., Singer, R. J., Edwards, P. P., J. Chem. Soc., Chem. Comm., 914 (1991); P. A. Anderson and P. P. Edwards, ibid., 915 (1991).
6. Anderson, P. A. and Edwards, P. P., J. Am. Chem. Soc. 114, 10608 (1992).
7. Edwards, P. P., Woodall, L. J., Anderson, P. A., Armstrong, A. R., Slaski, M., Chem. Soc. Rev. 22, 305 (1993).
8. Anderson, P. A., Edwards, P. P., Phys. Rev. B 50, 7155 (1994).
9. Waldram, J. R., Porch, A. and Cheah, H.-M., Physica C 232, 189 (1994).

Towards the Synthesis of Atomic Scale Wires

  • P. A. Anderson (a1), L. J. Woodall (a1), A. Porch (a2), A. R. Armstrong (a1), I. Hussain (a1) and P. P. Edwards (a1)...

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