Analysis of aerosols by LIBS

Ulrich Panne; David Hahn

doi:10.1017/CBO9780511541261.006

5 - Analysis of aerosols by LIBS

Published online by Cambridge University Press: 08 August 2009

Ulrich Panne and

David Hahn

Edited by

Andrzej W. Miziolek ,

Vincenzo Palleschi and

Israel Schechter

Show author details

Ulrich Panne: Affiliation:
Laboratory for Applied Laser Spectroscopy, Institute of Hydrochemistry, Technical University Munich
David Hahn: Affiliation:
Department of Mechanical and Aerospace Engineering, University of Florida
Andrzej W. Miziolek: Affiliation:
U.S. Army Research Laboratory, USA
Vincenzo Palleschi: Affiliation:
Istituto per I Processi Chimico-Fisici, Italy
Israel Schechter: Affiliation:
Technion - Israel Institute of Technology, Haifa

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Summary

Introduction to aerosol science

Fundamentals of aerosols

Laser-induced breakdown spectroscopy (LIBS) is well suited for the analysis of aerosol particles because of the unique point sampling nature of the laser-induced plasma. The discrete plasma volume uniquely couples with the discrete nature of aerosol particles to enable a wide range of data analysis options, including spectral averaging, conditional spectral processing, and single-shot analysis. In this chapter, a detailed introduction to aerosol science and aerosol analysis is presented to frame the overall problem of LIBS-based aerosol analysis. A detailed analysis of the laser-induced breakdown process is focused on the gas-phase processes associated with plasma initiation and propagation. Quantitative aerosol analysis is presented in terms of the aerosol-sampling problem, followed by direct and indirect quantitative aerosol measurements. We conclude with a detailed discussion of LIBS applications to aerosol analysis and future directions in this challenging and important area.

Aerosols (Latin, Aer (air) and sole (solutions)) are particle ensembles of solid and/or liquid matter with characteristic dimensions in the nanometer to micrometer range suspended in a gaseous carrier gas. Common usage, however, refers to aerosols often only as the particulate component. For many processes involving semivolatile components, the gas phase is, however, inextricably linked to the particle composition. In relation to their number density, aerosols are ubiquitous; however, the mass of a single aerosol particle is often negligibly small. For example, a solid spherical particle of 100 nm diameter with a density of 2 g cm−3 has a total mass of 1 fg.

Type: Chapter
Information: Laser Induced Breakdown Spectroscopy , pp. 194 - 253

DOI: https://doi.org/10.1017/CBO9780511541261.006 [Opens in a new window]

Publisher: Cambridge University Press

Print publication year: 2006

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5 - Analysis of aerosols by LIBS

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