Hostname: page-component-76fb5796d-zzh7m Total loading time: 0 Render date: 2024-04-26T08:54:26.592Z Has data issue: false hasContentIssue false

Onset of magnetic interface exchange interactions in epitaxially grown Mn/Co(001)

Published online by Cambridge University Press:  03 March 2011

J.T. Kohlhepp*
Affiliation:
Eindhoven University of Technology, Department of Applied Physics and Center for NanoMaterials (CNM), 5600MB Eindhoven, The Netherlands
H. Wieldraaijer
Affiliation:
Eindhoven University of Technology, Department of Applied Physics and Center for NanoMaterials (CNM), 5600MB Eindhoven, The Netherlands
W.J.M de Jonge
Affiliation:
Eindhoven University of Technology, Department of Applied Physics and Center for NanoMaterials (CNM), 5600MB Eindhoven, The Netherlands
*
a) Address all correspondence to this author. e-mail: j.t.kohlhepp@tue.nl This paper was selected as the Outstanding Meeting Paper for the 2006 MRS Spring Meeting Symposium Q Proceedings, Vol. 941E.
Get access

Abstract

Manganese (Mn) grows in a metastable expanded (c/a > 1) face-centered-tetragonal (fct) phase on thin fct-Co(001) template films. A layer-by-layer growth mode is observed for small Mn thicknesses. Antiferromagnetism (AFM) of fct-Mn is evidenced by the observation of shifted magnetization loops antiparallel to the cooling field direction (negative bias) and enhanced coercive fields for Co/Mn bilayers. At low temperature, magnetic exchange interactions are detected at the Co/Mn interface for nominal Mn thicknesses as low as 1.4 monolayer (ML), indicating the onset of AFM in 2-ML-thick Mn islands. However, between 2- and 5-ML Mn, a positive bias of the magnetization loops is observed in a certain temperature range below the blocking temperature (TB) of the films. This peculiar behavior is explained by the dependence of TB on both the local Mn ML thickness and the Mn island size, leading to a unidirectional coercivity enhancement in a temperature range where both blocked and unblocked regions coexist in the Mn layers.

Type
Outstanding Meeting Papers
Copyright
Copyright © Materials Research Society 2007

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

REFERENCES

1Nogués, J. and Schuller, I.K.: Exchange bias. J. Magn. Magn. Mater. 192, 203 (1999).CrossRefGoogle Scholar
2Berkowitz, A.E. and Takano, K.: Exchange anisotropy—A review. J. Magn. Magn. Mater. 200, 552 (1999).CrossRefGoogle Scholar
3Nogués, J., Sort, J., Langlais, V., Skumryev, V., Suriñach, S., Muñoz, J.S., and Baró, M.D.: Exchange bias in nanostructures. Phys. Rep. 422, 65 (2005).CrossRefGoogle Scholar
4Hafner, J. and Spišák, D.: Ab initio investigation of the magnetism of tetragonal Mn: Bulk, surface, ultrathin films, and multilayers. Phys. Rev. B 72, 144420 (2005).CrossRefGoogle Scholar
5Kohlhepp, J.T. and de Jonge, W.J.M.: Stabilization of metastable expanded face-centered-tetragonal manganese. Phys. Rev. Lett. 96, 237201 (2006).CrossRefGoogle ScholarPubMed
6Schmid, A.K. and Kirschner, J.: In situ observation of epitaxial growth of Co thin films on Cu(100). Ultramicroscopy 42, 483 (1992).CrossRefGoogle Scholar
7Wieldraaijer, H., de Jonge, W.J.M., and Kohlhepp, J.T.: Monolayer resolved oscillating hyperfine fields in epitaxial face-centered-tetragonal Co(001) films. Phys. Rev. Lett. 93, 177205 (2004).CrossRefGoogle ScholarPubMed
8Wieldraaijer, H., de Jonge, W.J.M., and Kohlhepp, J.T.: Electric-field gradients in thin face-centered-tetragonal Co films observed by nuclear magnetic resonance. Phys. Rev. B 72, 155409 (2005).CrossRefGoogle Scholar
9O’Brien, W.L. and Tonner, B.P.: Surface-enhanced magnetic moment and ferromagnetic ordering of Mn ultrathin films on fcc Co(001). Phys. Rev. B 50, 2963 (1994).CrossRefGoogle Scholar
10Leighton, C., Nogués, J., Jönsson-Åkerman, B.J., and Schuller, I.K.: Coercivity enhancement in exchange biased systems driven by interfacial magnetic frustration. Phys. Rev. Lett. 84, 3466 (2000).CrossRefGoogle ScholarPubMed
11Gredig, T., Krivorotov, I.N., Eames, P., and Dahlberg, E.D.: Unidirectional coercivity enhancement in exchange-biased Co/CoO. Appl. Phys. Lett. 81, 1270 (2002).CrossRefGoogle Scholar