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Preparation and enhanced off-resonance optical nonlinearities of CdS-capped gold nanoparticles embedded in BaTiO3 thin films

Published online by Cambridge University Press:  31 January 2011

Yong Yang
Affiliation:
State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, 200050, People's Republic of China
Jianlin Shi*
Affiliation:
State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, 200050, People's Republic of China
Hangrong Chen
Affiliation:
State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, 200050, People's Republic of China
Shugang Dai
Affiliation:
State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, 200050, People's Republic of China
Weiming Huang
Affiliation:
State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, 200050, People's Republic of China
Ye Liu
Affiliation:
Physics Department, National Key Laboratory of Applied Surface Physics, Fudan University, Shanghai, People's Republic of China
*
a) Address all correspondence to this author. e-mail: jlshi@sunm.shcnc.ac.cn
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Abstract

A simple approach has been developed for the synthesis of Au@CdS core-shell nanoparticles by a direct self-assembling process. Stable Au@CdS composite colloids were prepared by thiourea, as a double-functional reagent that acted as the linkage agent between Cd2+ ions and gold nanoparticles. The CdS-capped gold composite nanoparticles were successfully integrated into BaTiO3 films. A significant enhancement of third-order nonlinear optical susceptibility in the Au@CdS nanoparticles with core-shell structure is reported. To compare the effect of enhanced nonlinear response, single gold or CdS nanoparticles embedded in BaTiO3 films were also prepared.

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Articles
Copyright
Copyright © Materials Research Society 2002

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Preparation and enhanced off-resonance optical nonlinearities of CdS-capped gold nanoparticles embedded in BaTiO3 thin films
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