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Charge carrier trapping in highly-ordered lyotropic chromonic liquid crystal films based on ionic perylene diimide derivatives

Published online by Cambridge University Press:  25 November 2014

Pavlo V. Soroka ,
Alexander Yu. Vakhnin ,
Yuriy A. Skryshevskiy ,
Oleksandr P. Boiko ,
Maksim I. Anisimov ,
Yuriy L. Slominskiy ,
Vassili G. Nazarenko ,
Jan Genoe  and
Andrey Kadashchuk
Pavlo V. Soroka
Affiliation:
Institute of Physics, National Academy of Sciences of Ukraine, Prospect Nauky 46, 03028 Kyiv, Ukraine
Alexander Yu. Vakhnin
Affiliation:
Institute of Physics, National Academy of Sciences of Ukraine, Prospect Nauky 46, 03028 Kyiv, Ukraine
Yuriy A. Skryshevskiy
Affiliation:
Institute of Physics, National Academy of Sciences of Ukraine, Prospect Nauky 46, 03028 Kyiv, Ukraine
Oleksandr P. Boiko
Affiliation:
Institute of Physics, National Academy of Sciences of Ukraine, Prospect Nauky 46, 03028 Kyiv, Ukraine Center for Physical Sciences and Technology, Savanoriu 231, LT-02300 Vilnius, Lithuania
Maksim I. Anisimov
Affiliation:
Institute of Physics, National Academy of Sciences of Ukraine, Prospect Nauky 46, 03028 Kyiv, Ukraine
Yuriy L. Slominskiy
Affiliation:
Institute of Organic Chemistry, National Academy of Sciences of Ukraine, Murmanska 5, 02660 Kyiv, Ukraine
Vassili G. Nazarenko
Affiliation:
Institute of Physics, National Academy of Sciences of Ukraine, Prospect Nauky 46, 03028 Kyiv, Ukraine
Jan Genoe
Affiliation:
IMEC, Kapeldreef 75, B-3001 Leuven, Belgium
Andrey Kadashchuk*
Affiliation:
Institute of Physics, National Academy of Sciences of Ukraine, Prospect Nauky 46, 03028 Kyiv, Ukraine IMEC, Kapeldreef 75, B-3001 Leuven, Belgium
*
ae-mail: kadash@iop.kiev.ua
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Abstract

Charge carrier trapping in thin films of lyotropic chromonic liquid crystals (LCLCs) based on ionic perylene diimide derivative and in chemically-similar neutral N,N′-dipentyl-3,4,9,10-perylene-dicarboximide (PTCDI-C5) films is investigated by thermally-stimulated luminescence (TSL) technique. The LCLC films comprise elongated molecular aggregates featuring a long-range orientational order. The obtained results provide direct evidence for the improved energetic ordering (smaller effective energetic disorder) in aggregated LCLC films as compared to conventional PTCDI-C5 films. The width of the density-of-state distribution of 0.09 eV and 0.13 eV was estimated for the LCLC and PTCDI-C5 films, respectively. Relatively small effective energetic disorder in LCLC films is ascribed to formation of macroscopically larger LCLC aggregates.

Type
Research Article
Information
The European Physical Journal - Applied Physics , Volume 68 , Issue 3 , December 2014 , 30201
Copyright
© EDP Sciences, 2014

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