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Rubrene Single-crystal Organic Field Effect Transistor with Laser Ablated BaTiO3 Epitaxial Growth Thin-film as High-k Insulator

Published online by Cambridge University Press:  26 February 2011

Nobuya Hiroshiba
Affiliation:
hiro48n@sspns.phys.tohoku.ac.jp, Tohoku University, Department of Physics, 6-3 Aoba, Aramaki, Aoba, Sendai, 980-8578, Japan, +91-22-795-6468, +91-22-795-6470
Ryotaro Kumashiro
Affiliation:
rkuma@sspns.phys.tohoku.ac.jp, Tohoku University, Department of Physics, 6-3 Aoba, Aramaki, Aoba, Sendai, 980-8578, Japan
Taishi Takenobu
Affiliation:
takenobu@imr.tohoku.ac.jp, Tohoku University, IMR, Sendai, 980-8578, Japan
Naoya Komatsu
Affiliation:
komatsu@sspns.phys.tohoku.ac.jp, Tohoku University, Department of Physics, 6-3 Aoba, Aramaiki, Aoba, Sendai, 980-8578, Japan
Yusuke Suto
Affiliation:
suto@sspns.phys.tohoku.ac.jp, Tohoku University, Department of Physcis, 6-3 Aoba, Aramaki, Aoba, Sendai, 980-8578, Japan
Yoshihiro Iwasa
Affiliation:
iwasa@imr.tohoku.ac.jp, Tohoku University, IMR, Sendai, 980-8578, Japan
Kenta Kotani
Affiliation:
kenta@ile.osaka-u.ac.jp, Osaka University, Osaka, 565-0871, Japan
Iwao Kawayama
Affiliation:
kawayama@ile.osaka-u.ac.jp, Osaka University, Osaka, 565-0871, Japan
Masayoshi Tonouchi
Affiliation:
tonouchi@ile.osaka-u.ac.jp, Osaka University, Osaka, 565-0871, Japan
Katsumi Tanigaki
Affiliation:
tanigaki@sspns.phys.tohoku.ac.jp, Tohoku University, Department of Physics, 6-3 Aoba, Aramaki, Aoba, Sendai, 980-8578, Japan
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Abstract

High quality BaTiO3 thin film epitaxially grown on a Nb-doped SrTiO3 (BTO/Nb-STO) substrate by a laser ablation technique is employed as a high-k gate insulator for a field-effect transistor of a rubrene single crystal in order to search for the possibility of high carrier accumulation. The high dielectric constant of 280 esu for the prepared BaTiO3 thin film accumulates 0.1 holes/rubrene-molecule, which is 2.5 times as high as the maximum carrier number of 0.04 holes/rubrene-molecule attained in the case of SiO2 gate insulator. Important parameters of rubrene single crystal FETs on BTO/Nb- STO are also described in comparison with those on SiO2/doped-Si.

Type
Research Article
Copyright
Copyright © Materials Research Society 2007

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References

REFERENCES

1. Dimitrakopoulos, C. D. and Malenfant, P. R. L., Adv. Mater. 14, 99 (2002)Google Scholar
2. Jang, Y. et al., Appl. Phys. Lett. 87, 152105 (2005)Google Scholar
3. Abe, Y. et al., Appl. Phys. Lett. 87, 153506 (2005)Google Scholar
4. Boer, B. de et al., Adv. Mater. 17, 621 (2005)Google Scholar
5. Hiroshiba, N. et al., Chem. Phys. Lett. 400, 235 (2004)Google Scholar
6. Dimitrakopoulos, C. D., Purushothaman, S., Kymissis, J., Callegari, A., Shaw, J. M., Science 283, 822 (1999).Google Scholar
7. Stassen, A. F., Boer, R. W. I. de, Iosad, N. N., and Morpurgo, A. F., Appl. Phys. Lett. 85, 3899 (2004).Google Scholar
8. Kubozono, Y., Nagano, T., Haruyama, Y., Kuwahara, E., Takayanagi, T., Ochi, K., and Fujiwara, A. Appl. Phys. Lett. 87, 143506 (2005).Google Scholar
9. Takeya, J., Goldmann, C., Haas, S., Pernstich, K. P., Ketterer, B., and Batlogg, B., J. Appl. Phys. 94, 5800 (2003).Google Scholar
10. Kawayama, Iwao, Kotani, Kenta and Tonouchi, Masayoshi, Jpn. J. Appl. Phys., 41, 68036805 (2002)Google Scholar
11. Shimotani, H., Kanbara, T., Iwasa, Y., Tsukagoshi, K., Aoyagi, Y., Kataura, H., Appl. Phys. Lett. 88, 073104 (2006).Google Scholar