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The Redistribution of Uranium Series Radionuclides at Koongarra

Published online by Cambridge University Press:  28 February 2011

Robert Edis*
Affiliation:
Australian Nuclear Science and Technology Organisation, Lucas Heights Research Laboratories, PMB 1, MENAI NSW 2234, AUSTRALIA.
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Abstract

The distribution of 238U, 234U, 230Th and 236Ra in rocks from the Koongarra uranium deposit has been examined. Alpha-spectrometry and ICP-MS were used to estimate elements in “accessible” and “inaccessible” phases, separated by a two-phase extraction scheme; and bulk analyses of visibly distinct zones were made using PIXE-PIGME, DNAA and XRF.

The secondary U dispersion fan of the Koongarra site is characterised by 234U/238U, 230Th/234U and 236Ra/230Th activity ratios (ARs) below unity in the extractable (accessible) phases, and above unity in the non-extractable (inaccessible) phases. The patterns of the ARs suggest zones of different U deposition and leaching rates with the most rapid accumulation at the base of weathering, especially at the extremities of the dispersion fan.

Type
Research Article
Copyright
Copyright © Materials Research Society 1991

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References

REFERENCES

1 Alligator Rivers Analogue Project, 1st Annual Report 1988-1989, edited by Duerden, P, 1990.Google Scholar
2 Snelling, A, Koongarra Uranium Deposit, in The Geology of the Mineral Deposits of Australia and Papua New Guinea, edited by Hughes, F E (Australasian Institute of Mining & Metallurgy, Melbourne, Monograph 14, 1989).Google Scholar
3 Yanase, N, Nightingale, T, Payne, T and Duerden, P, Uranium Distribution in Adsorbed and Mineral Phases of Rock by Sequential Extraction Method, Proceedings of Migration 89 (in press) (1989).Google Scholar
4 Lowson, R T, Short, S A, Davey, B G and Gray, D J, 234U/238U and 230Th/234U Activity Ratios in Mineral Phases of a Lateritic Weathered Zone. Geochim. Cosmochim. Acta 50, 16971702 (1986).Google Scholar
5 Nightingale, T, Mobilisation and Redistribution of Radionuclides during Weathering of a Uranium Ore body. MSc Thesis, University of Sydney (1988).Google Scholar
6 Edghill, R, The Redistribution of Uranium with Weathering in the Koongarra Uranium Deposit, Proceedings of Migration 89, (in press) (1989).Google Scholar
7 Murakami, T, Isobe, H and Edis, R, Effects of Chlorite Alteration on Uranium Redistribution in Koongarra, Australia, Uranium Series Nuclides Migration, 1990 MRS Fall Meeting, Boston (to be published).Google Scholar
8 Payne, T, in Alligator Rivers Analogue Project, Progress Report, 1 December 1989-28 February 1990, edited by Duerden, P, 1990.Google Scholar