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One-Year Leaching of Three SRL Glasses in Granite

Published online by Cambridge University Press:  26 February 2011

Bing-Fu Zhu
Affiliation:
Department of Materials Science and Engineering, University of Florida, Gainesville, FL 32611
D. E. Clark
Affiliation:
Department of Materials Science and Engineering, University of Florida, Gainesville, FL 32611
L. L. Hench
Affiliation:
Department of Materials Science and Engineering, University of Florida, Gainesville, FL 32611
G. G. Wicks
Affiliation:
E.I. du Pont de Nemours & Co., Savannah River Laboratory, Aiken, SC 29808
Lars Werme
Affiliation:
Swedish Nuclear Fuel Supply Co. (SKBF/KBS), P.O. Box 5864, S-102, Stockholm, Sweden
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Abstract

Three Savannah River Laboratory (SRL) simulated nuclear waste glasses were buried in granite boreholes 345 meters deep. Included in the same boreholes were other potential waste package components including stainless steel and bentonite. Samples were maintained at either ambient mine temperature (8–10°C) or 90°C. Differences in glass leaching performances were observed among the three compositions, with SRL 165 being more durable than SRL 131, both with 29.8% TDS waste. Likewise, the presence of some package components affected the leaching performances. Bentonite resulted in accelerated attack on the glass while the presence of stainless steel did not appear to have much effect. Results obtained through one year of burial are presented in this paper.

Type
Research Article
Copyright
Copyright © Materials Research Society 1985

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References

1. Nogues, T.L., Hench, L.L. and Zarsycki, J., “Comparative Study of Seven Glasses for Solidification of Nuclear Wastes,” in Scientific Basis for Nuclear Waste Management, V., Lutze, W., Ed., Elsevier Science Pub. Co., 1982.Google Scholar
2. Hench, L.L., “Glass Surfaces – 1982,” Proceedings of Int. Conf. on Physics of Amorphous Solids, Montpellier, France, July 1982, Zarzycki, J., Ed.CrossRefGoogle Scholar
3. Clark, D.E., Zhu, B.F. and Wicks, G.G., “Nuclear Waste Glass Leaching – Comparison of Laboratory and Field Tests,” presented at 1984 Int. Symposium on Glass, Beijing, Sept. 1984, to be published in the Symposium Proceedings.Google Scholar
4. Clark, D.E., Zhu, B.F., Robinson, R.S. and Wicks, G.G., “Preliminary Report on a Glass Burial Experiment in Granite,” Nuclear Waste Management, Advances in Ceramics, Vol.8, Wicks, G.G. and Ross, W.A., Ed., AcerS Inc., Columbus, Ohio 1984.Google Scholar
5. Grambow, B., “The Role of Metal Ion Solubility,” in Scientific Basis for Nuclear Waste Management V., Lutze, W., Ed., Elsevier Science Pub. Co., 1982.Google Scholar
6. PNL-5157, UC-70, “Final Report of the Defense High Level Waste Leaching Mechanisms Program,” p. 141, August 1984.Google Scholar