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Non-Linear Optical Response of Metallic and Emiconducting Nanocrystals in Fused Silica

Published online by Cambridge University Press:  03 September 2012

R. G. Elliman
Affiliation:
Electronic Materials Engineering Department
B. Luther-Davies
Affiliation:
Laser Physics Centre, R.S.Phys.S.E., Institute of Advanced Study, Australian National University, Canberra, ACT 0200.
M. Samoc
Affiliation:
Laser Physics Centre, R.S.Phys.S.E., Institute of Advanced Study, Australian National University, Canberra, ACT 0200.
A. Dowd
Affiliation:
Electronic Materials Engineering Department
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Abstract

The linear and nonlinear optical properties of Ge-implanted fused-silica were examined and compared with Au- and Si-implanted samples. Samples as-implanted with 1.0 MeV Ge ions to a fluence of 3x1017 Ge.cm-2 exhibited relatively large non-linearities, |n2| ≤5x10-12 cm2/W, and fast relaxation times, ∼lps. In contrast, samples implanted with comparable fluences of Au ions exhibited smaller non-linearities, |n2| ∼1x10-13 cm2/W, and slower response times, ≥ 10ps. The non-linearity for Ge was much larger than that for samples as-implanted with Si.

Type
Research Article
Copyright
Copyright © Materials Research Society 1997

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