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Nonlinear Optical Properties of Polyenes: Electron Correlation and Chain Conformation†

Published online by Cambridge University Press:  25 February 2011

A. F. Garito ,
J. R. Heflin ,
K. Y. Wong  and
O. Zamani-Khamiri
A. F. Garito
Affiliation:
Department of Physics and Laboratory for Research on the Structure of Matter, University of Pennsylvania, Philadelphia, PA 19104
J. R. Heflin
Affiliation:
Department of Physics and Laboratory for Research on the Structure of Matter, University of Pennsylvania, Philadelphia, PA 19104
K. Y. Wong
Affiliation:
Department of Physics and Laboratory for Research on the Structure of Matter, University of Pennsylvania, Philadelphia, PA 19104
O. Zamani-Khamiri
Affiliation:
Department of Physics and Laboratory for Research on the Structure of Matter, University of Pennsylvania, Philadelphia, PA 19104
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Abstract

Using a recently developed many-electron theory of second and third order nonlinear optical susceptibilities, microscopic descriptions of γxxxx(-3ω;ω,ω,ω) are presented for two conformations of polyenes. The importance of electron correlations and the effects of variation in conformation and chain length are discussed.

Type
Research Article
Information
MRS Online Proceedings Library (OPL) , Volume 109: Symposium K – Nonlinear Optical Properties of Polymers , 1987 , 91
Copyright
Copyright © Materials Research Society 1988

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Footnotes

†

Presented in part in the XV International Quantum Electronics Confrence, Baltimore, April 1987.

References

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