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Synthesis and photoluminescent properties of nanoerythrocyte-shaped ytterbium orthovanadate and erbium ion-doped ytterbium orthovanadate powders

Published online by Cambridge University Press:  06 March 2013

Youjin Zhang ,
Hongmei He ,
Ao Zheng  and
Yun Fan
Youjin Zhang*
Affiliation:
Department of Chemistry, University of Science and Technology of China, Hefei, 230026, People’s Republic of China
Hongmei He
Affiliation:
Department of Chemistry, University of Science and Technology of China, Hefei, 230026, People’s Republic of China
Ao Zheng
Affiliation:
Department of Chemistry, University of Science and Technology of China, Hefei, 230026, People’s Republic of China
Yun Fan
Affiliation:
Department of Chemistry, University of Science and Technology of China, Hefei, 230026, People’s Republic of China
*
a)Address all correspondence to this author. e-mail: zyj@ustc.edu.cn
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Abstract

Nanoerythrocyte-shaped ytterbium orthovanadate (YbVO4) with substantially uniform size have been successfully synthesized by a simple and facile trisodium citrate-assisted hydrothermal method. The erythrocyte-shaped YbVO4 nanocrystals with self-assembled spherical and biconcave structure have a diameter of ∼500 nm, which were characterized by x-ray diffraction, x-ray photoelectron spectroscopy, Fourier transform infrared spectroscopy, field-emission scanning electron microscopy, high-resolution transmission electron microscopy and photoluminescence. The luminescent properties of erbium ion-doped ytterbium orthovanadate nanocrystals with different morphologies by different complexing agents were different in the relative intensity under identical measurement conditions, which exhibited the interesting morphology-dependent optical properties. The different energy transfer mechanisms and photoluminescence intensities might be the result of the greatly reduced defect centers.

Keywords

optical propertieshydrothermalmorphology
Type
Articles
Information
Journal of Materials Research , Volume 28 , Issue 6 , 28 March 2013 , pp. 856 - 862
Copyright
Copyright © Materials Research Society 2013

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