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In-Situ Radiocarbon Production by Neutrons and Muons in an Antarctic Blue Ice Field at Scharffenbergbotnen: A Status Report

Published online by Cambridge University Press:  18 July 2016

K van der Borg*
Affiliation:
Institute of Subatomic Physics, Faculty of Physics and Astronomy, Utrecht University, P.O. Box 80000, 3508 TA Utrecht, The Netherlands
W J M van der Kemp
Affiliation:
Institute of Subatomic Physics, Faculty of Physics and Astronomy, Utrecht University, P.O. Box 80000, 3508 TA Utrecht, The Netherlands
C Alderliesten
Affiliation:
Institute of Subatomic Physics, Faculty of Physics and Astronomy, Utrecht University, P.O. Box 80000, 3508 TA Utrecht, The Netherlands
A F M de Jong
Affiliation:
Institute of Subatomic Physics, Faculty of Physics and Astronomy, Utrecht University, P.O. Box 80000, 3508 TA Utrecht, The Netherlands
R A N Lamers
Affiliation:
Institute of Subatomic Physics, Faculty of Physics and Astronomy, Utrecht University, P.O. Box 80000, 3508 TA Utrecht, The Netherlands
J Oerlemans
Affiliation:
Institute of Marine and Atmospheric Research, Faculty of Physics and Astronomy, Utrecht University, P.O. Box 80005, 3508 TA Utrecht, The Netherlands
M Thomassen
Affiliation:
Institute of Marine and Atmospheric Research, Faculty of Physics and Astronomy, Utrecht University, P.O. Box 80005, 3508 TA Utrecht, The Netherlands
R S W van de Wal
Affiliation:
Institute of Marine and Atmospheric Research, Faculty of Physics and Astronomy, Utrecht University, P.O. Box 80005, 3508 TA Utrecht, The Netherlands
*
Corresponding author. Email: k.vanderborg@phys.uu.nl.
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Abstract

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In the radiocarbon accelerator mass spectrometry (14C AMS) analysis of gases obtained in a dry extraction from a 52–m Antarctic ice core, we observed 14CO2 and 14CO concentrations decreasing with depth. The concentrations are explained in terms of in-situ production by neutrons and captured muons in ablating ice. The ratio of the 14CO2 concentration to that of 14CO has been found to be constant at 1.9 ± 0.3. The ablation rates obtained of 42 ± 18 cm.yr−1 and 40 ± 13 cm.yr−1 for the neutron and muon components, respectively, are about three times higher than observed from stake readings. The discrepancy may point to an incomplete extraction of the dry extraction method. Using the constant ratio in 14CO2 and 14CO concentrations we correct for the in-situ component in the trapped 14CO2 and deduce an age of 10,300 ± 900 BP for the ice core.

Type
I. Our ‘Dry’ Environment: Above Sea Level
Copyright
Copyright © 2001 by the Arizona Board of Regents on behalf of the University of Arizona 

References

Alderliesten, C, van der Borg, K, de Jong, AFM. 1997. Contamination and fractionation effects in AMS-measured 14C/14C and 14C/14C ratios of small samples. Radiocarbon 40(2):215–21.Google Scholar
Andreé, M, Moor, E, Beer, J, Oeschger, H, Bonani, G, Hoffman, HJ, Morenzoni, E, Nessi, M, Suter, M, Wölfli, W. 1984. 14C dating of polar ice. Nuclear Instruments and Methods in Physics Research B5:385–8.Google Scholar
Bilokon, H, Cini Castagnoli, G, Castellina, A, D'Ettore Piazolli, B, Mannochini, G, Meroni, E, Picchi, P, Vernetto, S. 1989. Flux of vertical negative muons stopping at depths 0.35 – 1000 hg/cm2 . Journal of Geophysics Research 94:145–52.Google Scholar
Brown, ET, Bourles, DL, Colin, F, Raisbeck, GM, Yiou, F, Desgarceaux, S. 1995. Evidence for muon-induced production of 10Be in near-surface rocks from the Congo. Geophysical Research Letters 22(6):703–6.Google Scholar
Cassidy, W, Harvey, R, Schutt, J, Delisle, G, Yanai, K. 1992. The meteorite collection sites of Antarctica. Meteoritics 27:490525.CrossRefGoogle Scholar
von Egidy, T, Hartmann, FJ. 1982. Average muonic Coulomb capture probabilities for 65 elements. Physical Review A26:2355–60.Google Scholar
Fireman, EL, Norris, TL. 1982. Ages and composition of gas trapped in Allan Hills and Byrd core ice. Earth and Planetary Science Letters 60:339–50.Google Scholar
Heisinger, BP. 1998. Myonen-induzierte Production von Radionukliden [thesis]. München: Technical University. Unpublished.Google Scholar
Jonsson, S. 1992. Local climate and mass balance of a blue-ice area in Western Dronning Maud Land, Antarctica. Zeitschrift für Gletscherkunde und Glaciologie 26:1129.Google Scholar
Jouzel, J, Lorius, C, Petit, JR, Genthon, C, Barkov, NI, Kotyakov, VM, Petrov, VN. 1987. Vostok ice core: a continuous isotope temperature record over the last climatic cycle (160,000 years). Nature 329:403–8.CrossRefGoogle Scholar
Jull, AJT, Lal, D, Donahue, DJ, Mayewski, P, Lorius, C, Raynaud, D, Petit, JR. 1994. Measurements of cosmic-ray produced 14C in firn and ice from Antarctica. Nuclear Instruments and Methods in Physics Research B92:326–30.Google Scholar
Kubik, PW, Korschinek, G, Nolte, E, Ratzinger, U, Ernst, H, Teichmann, S, Morinaga, H. 1994. Accelerator mass spectrometry of 36C1 in limestone and some paleontological samples using completely stripped ions. Nuclear Instruments and Methods in Physics Research B5:326–30.Google Scholar
Lal, D, Peters, B. 1967. Cosmic-ray produced radioactivity on the earth. In: Handbuch der physik. Volume 46/2. Berlin: Springer-Verlag, p 551612.Google Scholar
Lal, D, Nishiizumi, K, Arnold, JR. 1987. In situ cosmogenic 14C, 10Be, and 26Al for determining the net accumulation and ablation rates of ice sheets. Journal of Geophysical Research 92(B6):4947–52.Google Scholar
Lal, D, Jull, AJT, Donahue, DJ, Burtner, D, Nishiizumi, . 1990. Polar ice ablation rates measured using in situ cosmogenic 14C. Nature 346:350–2.Google Scholar
Lal, D. 1991. Cosmic ray labelling of erosion surfaces: in situ nuclide production rates and erosion models. Earth and Planetary Science Letters 104:424–39.CrossRefGoogle Scholar
Lal, D, Jull, AJT, Donahue, DJ, Burr, GS, Deck, B, Jouzel, J, Steig, E. 2000. The record of cosmogenic in-situ produced 14C in Vostok and Taylor Dome ice samples: implications to strong role of wind ventilation processes. Journal of Geophysical Research Forthcoming.Google Scholar
Lambrecht, RM. 1997. Evidence for insertion mode reaction of energetic carbon-11 with oxygen. Radiochimica Acta 77:3743.Google Scholar
Lifton, NA, Jull, AJT, Quade, J. 2000. A new extraction technique and production rate estimate for in situ cosmogenic 14C in quartz. Radiocarbon. Submitted.Google Scholar
Raynaud, D, Jouzel, J, Barnola, JM, Chappallaz, J, Delmas, RJ, Lorius, C. 1993. The ice record of greenhouse gases. Science 259:926–34.Google Scholar
Schwander, J, Stauffer, B. 1984. Age differences between polar ice and the air trapped in the bubbles. Nature 311:45–7.Google Scholar
van der Borg, K, Alderliesten, C, Houston, CM, de Jong, AFM, van Zwol, NA. 1987. Accelerator mass spectrometry with 14C and 10Be in Utrecht. Nuclear Instruments and Methods in Physics Research B29:143–5.Google Scholar
van der Borg, K, Alderliesten, C, de Jong, AFM, van den Brink, A, de Haas, AP, Kersemaekers, HJH, Raaymakers, JEMJ. 1997. Precision and mass fractionation in 14C analysis with AMS. Nuclear Instruments and Methods in Physics Research B123:97101.Google Scholar
van der Kemp, WJM, Alderliesten, C, van der Borg, K, Holmlund, P, de Jong, AFM, Karlöf, L, Lamers, RAN, Oerlemans, J, Thomassen, M, van der Wal, RSW. 2000. Very little in-situ produced 14C retained in accumulating Antarctic ice. Nuclear Instruments and Methods in Physics Research B172:632–6.Google Scholar
van Roijen, JJ, van der Borg, K, de Jong, AFM, Oerlemans, J. 1995. A correction for in-situ 14C in Antarctic ice with 14CO. Radiocarbon 37(2):165–9.Google Scholar
van Roijen, JJ. 1996. Determination of ages and specific mass balances from 14C measurements on Antarctic surface ice [thesis]. Utrecht University. Unpublished.Google Scholar