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Micro- to Nano-scale Structure and Drug Release Behavior of Solutions and Hydrogels of Poly (lactide)-Poly (ethylene oxide)-Poly (lactide) Triblock Copolymers

Published online by Cambridge University Press:  26 February 2011

Sarvesh Kumar Agrawal
Affiliation:
sagrawal@ecs.umass.edu, University of Massachusetts, Amherst, Chemical Engineering, 686, North Pleasant Street, Amherst, MA, 01003, United States, 413-577-2593
Naomi Sanabria-DeLong
Affiliation:
naomisd@mail.pse.umass.edu, University of Massachusetts, Amherst, Polymer Science and Engineering, United States
Pete R. Jemian
Affiliation:
jemian@anl.gov, University of Illinois at Urbana-Champaign, Frederick Seitz Materials Research Laboratory, United States
Jeannine M. Coburn
Affiliation:
jmcoburn@student.umass.edu, University of Massachusetts, Amherst, Chemical Engineering, United States
Gregory N. Tew
Affiliation:
tew@mail.pse.umass.edu, University of Massachusetts, Amherst, Polymer Science and Engineering, United States
Surita R. Bhatia
Affiliation:
sbhatia@ecs.umass.edu, University of Massachusetts, Amherst, Chemical Engineering, United States
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Abstract

We have performed for the first time a complete structural characterization of PLA-PEO-PLA in the solution and hydrogel states. Previous studies on hydrogels of these polymers have shown that these gels have excellent mechanical properties suitable for possible application in tissue engineering and drug delivery. We have performed SANS, USAXS and confocal microscopy to relate the change in micro to nano scale self-assembled structure of these polymers in aqueous solution with changes in the block length and stereospecificity of the PLA block. A significant difference in structure and association behavior was seen between the polymers made from amorphous D/L-lactide as compared to those with crystalline L lactide blocks. In the former case spherical micelles were seen to form whereas the latter forms nonspherical polydisperse micellar assemblies. Both polymers form an associative network structure at higher concentrations, leading to gelation. USAXS and confocal microscopy show the presence of large-scale fractal aggregates in the hydrogels of these polymers. The fractal structure was denser for the L lactide series polymers as compared to the D/L-lactide series polymers. These results show that we can tune the microstructure and thereby the mechanical strength of these gels depending upon the specific application we need it for. We also show profiles for release of hydrophobic drug sulindac from 5 weight% solutions of these polymers in phosphate buffer saline. The profiles follows an almost zero order release behavior that continues slowly and steadily over several days and is again found to be strongly dependent on the crystallinity and molecular weight of the PLA block.

Type
Research Article
Copyright
Copyright © Materials Research Society 2006

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