Hostname: page-component-77c89778f8-7drxs Total loading time: 0 Render date: 2024-07-18T11:36:53.475Z Has data issue: false hasContentIssue false

Development of a New Mechanistic Low-Level Waste Source Term Model

Published online by Cambridge University Press:  03 September 2012

Man-Sung Yim*
Affiliation:
Department of Nuclear Engineering, North Carolina State University, Raleigh, NC 27695
Get access

Abstract

A new mechanistic low-level waste source term model was developed. Key features of this effort are: use of cumulative probability functions to describe the failures of waste containers; capability to describe diffusion controlled release which is dependent on the conditions of the waste package surroundings; consideration of the effects of gas generation on the source term, and; use of a source inventory characterization routine to provide a built-in capability for defining the distributions of radionuclides in various waste forms and streams. The model is capable of describing the diffusion of radionuclides in waste forms with the use of concentration and flux continuity boundary conditions. Release of radionuclides from various waste streams is modeled by the combination of diffusion, dissolution, and surface release. Failures of waste containers are portrayed by the use of probabilistic failure functions based on Weibull and lognormal distributions. The model for radionuclide release from waste packages is coupled with the near-field transport model to describe the effects of migration and dispersion within the disposal unit. Characteristics of the new model were evaluated through sensitivity analysis and compared with existing source term codes.

Type
Research Article
Copyright
Copyright © Materials Research Society 1997

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

REFERENCES

1. Bullen, D. B., “A Model for Container Performance in An Unsaturated Repository,” Nuclear Technology, Vol. 113, pp. 2945, 1996.Google Scholar
2. Sullivan, T. M. and Suen, S. J., “Low-Level Waste Shallow Land Disposal Source Term Model: Data Input Guides,” NUREG/CR-5387, U. S. Nuclear Regulatory Commission, 1989.Google Scholar
3. U.S. Nuclear Regulatory Commission, “Source Term Implementation for Initial Performance Assessment Calculation,” Technical Review of Performance Assessment Modeling Strategy, Rockville, MD, July 12–13, 1993.Google Scholar
4. Sullivan, T. M., “Selection of Models to Calculate the LLW Source Term,” NUREG/CR-5773, U. S. Nuclear Regulatory Commission, 1991.10.2172/6125438Google Scholar
5. Kim, C. L., Cho, C. H., and Choi, H. J., “Equilibrium Concentration and Diffusion Controlled Leaching Model for Cement-Based Waste Forms,” Waste Management, Vol. 15, no. 5/6, 1995.Google Scholar
6. Yim, M.-S. and Simonson, S. A., “Generation and Release of Radioactive Gases in LLW Disposal Facilities,” The 23rd DOE/NRC Nuclear Air Cleaning and Treatment Conference, NUREG/CP-0141, CONF-940738, 1995.10.2172/95643Google Scholar
7. Yim, M.-S., Simonson, S. A., and Sullivan, T. M., “Investigation of C-14 Release from a Generic Low-Level Waste Disposal Facility,” Nuclear Technology, Vol. 114, no. 2, 1996.10.13182/NT96-A35254Google Scholar
8. U.S. Nuclear Regulatory Commission, “Overview of NRC Staff LLWPA Modeling Efforts,” Low-Level Waste Performance Assessment Workshop, Rockville, MD, November 17, 1994.Google Scholar
9. Sullivan, T. M., “Disposal Unit Source Term (DUST) Data Input Guide,” NUREG/CR-6041, U. S. Nuclear Regulatory Commission, 1993.10.2172/10162170Google Scholar
10. Rogers, V. and Hung, C., “PRESTO-EPA-CPG: A Low-Level Radioactive Waste Environmental Transport and Risk Assessment Code, Documentation and User's Manual,”EPA 520/1–87–026, U. S. Environmental Protection Agency, 1987.Google Scholar