Hostname: page-component-7bb8b95d7b-cx56b Total loading time: 0 Render date: 2024-09-07T23:42:05.871Z Has data issue: false hasContentIssue false

Near-Field Optical Spectroscopy: Enhancing the Light Budget

Published online by Cambridge University Press:  02 July 2020

M.A. Paesler
Affiliation:
Physics Department, North Carolina State University, Raleigh, NC27695-8202, USA Institute of Applied Photophysics, Technical University Dresden, D-01069, Dresden, Germany
H.D. Hallen
Affiliation:
Physics Department, North Carolina State University, Raleigh, NC27695-8202, USA
B.I. Yakobson
Affiliation:
Physics Department, North Carolina State University, Raleigh, NC27695-8202, USA
C.J. Jahncke
Affiliation:
Physics Department, North Carolina State University, Raleigh, NC27695-8202, USA
P.O. Boykin
Affiliation:
Physics Department, North Carolina State University, Raleigh, NC27695-8202, USA
A. Meixner
Affiliation:
Institute of Applied Photophysics, Technical University Dresden, D-01069, Dresden, Germany
Get access

Extract

The near-field scanning optical microscope, or NSOM, provides spectroscopists with resolution beneath the diffraction limit. In the NSOM, an optical aperture smaller than the wavelength λ of the probe radiation is scanned in the near-field of a sample. Pixels are serially gathered and then constituted as a computer-generated image. Spectroscopic NSOM investigations demonstrating sub-λ, resolution include studies of photoluminescence, Raman spectroscopy, and single molecule fluorescence. Results of nano-Raman spectroscopy on semiconducting Rb-doped KTP are shown in figure 1. Figure la is a topographic image of the sample showing a square Rb-doped region in an otherwise undoped sample. Figure lc is a NSOM region of the corner of the doped region, and figure lb is an image of the same region taken within a Raman line. While these data do provide sub-λ spectroscopic resolution and other interesting features, the weak signal provided by current NSOM technologies and the low quantum efficiency of the Raman effect necessitated development of a very low-drift microscope and inconveniently long collection times.

Type
Optical Microanalysis
Copyright
Copyright © Microscopy Society of America 1997

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

1. Paesler, M.A. and Moyer, P.J., Near-field Optics:Theory, Instrumentation, and Applications, John Wiley & Sons, NY 1996.Google Scholar

2. Jahncke, C L. and Hallen, H.D., LEOS 96 conference proceedings vol. 1, pp. 176177.Google Scholar

3. LaRosa, A., Yakobson, B.I., and Hallen, H.D., Appl. Phys. Lett. 67 (18), 2597 (1995). Boykin, P.O. and Yakobson, B.I., Proc. SPIE 2677,148 (1996).Google Scholar

4. Buckland, E., Moyer, P.J. and Paesler, M.A., J. Appl. Phys., 73,1018 (1993).CrossRefGoogle Scholar

5. Research supported by US Army (DAAH04-93-G-164 and DAAH04-G-064) and NSF (DMR-9300041).Google Scholar