Kinetic modeling of laser-ion beam generation from the “break-out afterburner” (BOA) has been modeled for several deuteron-rich solid-density target foils. Modeling the transport of these beams in a beryllium converter shows as much as a fourfold increase in neutron yield over the present state of the art through the use of alternative target materials. Additionally, species-separation dynamics during the BOA can be exploited to control the hardness of the neutron spectra, of interest for, for example, enhancing penetrability in shielded material in active neutron interrogation settings.

The laser system PALS, as a driver of a broad-beam ion source, delivered deuterons which generated neutrons with energies higher than 14 MeV through the $\def \xmlpi #1{}\def \mathsfbi #1{\boldsymbol {\mathsf {#1}}}\let \le =\leqslant \let \leq =\leqslant \let \ge =\geqslant \let \geq =\geqslant \def \Pr {\mathit {Pr}}\def \Fr {\mathit {Fr}}\def \Rey {\mathit {Re}}{}^{7}\mathrm{Li(d,n)}{}^{8}\mathrm{Be}$ reaction. Deuterons with sub-MeV energy were accelerated from the front surface of a massive $\mathrm{CD}_{2}$ target in the backward direction with respect to the laser beam vector. Simultaneously, neutrons were emitted from the primary $\mathrm{CD}_{2}$ target and a secondary LiF catcher. The total maximum measured neutron yield from ${}^{2}\mathrm{D(d,n)}{}^{3}\mathrm{He}$, ${}^{7}\mathrm{Li(d,n)}{}^{8}\mathrm{Be}$, ${}^{12}\mathrm{C(d,n)}{}^{13}\mathrm{N}$ reactions was ${\sim } 3.5 ({\pm }0.5) \times 10^{8}\ \mathrm{neutrons/shot}$.