The interaction of relativistically intense lasers with opaque targets represents a highly non-linear, multi-dimensional parameter space. This limits the utility of sequential 1D scanning of experimental parameters for the optimization of secondary radiation, although to-date this has been the accepted methodology due to low data acquisition rates. High repetition-rate (HRR) lasers augmented by machine learning present a valuable opportunity for efficient source optimization. Here, an automated, HRR-compatible system produced high-fidelity parameter scans, revealing the influence of laser intensity on target pre-heating and proton generation. A closed-loop Bayesian optimization of maximum proton energy, through control of the laser wavefront and target position, produced proton beams with equivalent maximum energy to manually optimized laser pulses but using only 60% of the laser energy. This demonstration of automated optimization of laser-driven proton beams is a crucial step towards deeper physical insight and the construction of future radiation sources.

We present the development and characterization of a high-stability, multi-material, multi-thickness tape-drive target for laser-driven acceleration at repetition rates of up to 100 Hz. The tape surface position was measured to be stable on the sub-micrometre scale, compatible with the high-numerical aperture focusing geometries required to achieve relativistic intensity interactions with the pulse energy available in current multi-Hz and near-future higher repetition-rate lasers ( $>$ kHz). Long-term drift was characterized at 100 Hz demonstrating suitability for operation over extended periods. The target was continuously operated at up to 5 Hz in a recent experiment for 70,000 shots without intervention by the experimental team, with the exception of tape replacement, producing the largest data-set of relativistically intense laser–solid foil measurements to date. This tape drive provides robust targetry for the generation and study of high-repetition-rate ion beams using next-generation high-power laser systems, also enabling wider applications of laser-driven proton sources.

A machine learning model was created to predict the electron spectrum generated by a GeV-class laser wakefield accelerator. The model was constructed from variational convolutional neural networks, which mapped the results of secondary laser and plasma diagnostics to the generated electron spectrum. An ensemble of trained networks was used to predict the electron spectrum and to provide an estimation of the uncertainty of that prediction. It is anticipated that this approach will be useful for inferring the electron spectrum prior to undergoing any process that can alter or destroy the beam. In addition, the model provides insight into the scaling of electron beam properties due to stochastic fluctuations in the laser energy and plasma electron density.

Filamentary structures can form within the beam of protons accelerated during the interaction of an intense laser pulse with an ultrathin foil target. Such behaviour is shown to be dependent upon the formation time of quasi-static magnetic field structures throughout the target volume and the extent of the rear surface proton expansion over the same period. This is observed via both numerical and experimental investigations. By controlling the intensity profile of the laser drive, via the use of two temporally separated pulses, both the initial rear surface proton expansion and magnetic field formation time can be varied, resulting in modification to the degree of filamentary structure present within the laser-driven proton beam.

High-intensity femtosecond laser–plasma interaction experiments were performed to investigate laser–plasma wakefield acceleration in the “bubble” regime. Using a 15 TW laser pulse, the emission of side-scattered radiation was spectrally and spatially resolved and was consequently used to diagnose the evolution of the laser pulse during the acceleration process. Side-scattered emission was observed immediately before wavebreaking at a frequency of ωL + 1.7ωp (where ωL is the laser frequency and ωp is the background plasma frequency). This emission may result from scattering of laser light by large amplitude plasma oscillations generated in the shell of the wakefield “bubble” and which occurs immediately prior to the wavebreaking/injection process. The observed variation of the frequency of scattered light with electron density agrees with theoretical estimates.

We report on the experimental demonstration of a technique to generate steep density gradients in gas-jet targets of interest to laser–plasma ion acceleration. By using an intentional low-energy prepulse, we generated a hydrodynamic blast wave in the gas to shape the target prior to the arrival of an intense CO$_{2}$ (${\it\lambda}\approx 10~{\rm\mu}\text{m}$) drive pulse. This technique has been recently shown to facilitate the generation of ion beams by shockwave acceleration (Tresca et al., Phys. Rev. Lett., vol. 115 (9), 2015, 094802). Here, we discuss and introduce a model to understand the generation of these blast waves and discuss in depth the experimental realisation of the technique, supported by hydrodynamics simulations. With appropriate prepulse energy and timing, this blast wave can generate steepened density gradients as short as $l\approx 20~{\rm\mu}\text{m}$ ($1/e$), opening up new possibilities for laser–plasma studies with near-critical gaseous targets.

Experiments have shown that the ion energy obtained by laser–ion acceleration can be optimized by choosing either the appropriate pulse duration or the appropriate target thickness. We demonstrate that this behavior can be described either by the target normal sheath acceleration model of Schreiber et al. or by the radiation pressure acceleration model of Bulanov and coworkers. The starting point of our considerations is that the essential property of a laser system for ion acceleration is its pulse energy and not its intensity. Maybe surprisingly we show that higher ion energies can be reached with reduced intensities.

The energy transfer by stimulated Brillouin backscatter from a long pump pulse (15 ps) to a short seed pulse (1 ps) has been investigated in a proof-of-principle demonstration experiment. The two pulses were both amplified in different beamlines of a Nd:glass laser system, had a central wavelength of 1054 nm and a spectral bandwidth of 2 nm, and crossed each other in an underdense plasma in a counter-propagating geometry, off-set by $\def \xmlpi #1{}\def \mathsfbi #1{\boldsymbol {\mathsf {#1}}}\let \le =\leqslant \let \leq =\leqslant \let \ge =\geqslant \let \geq =\geqslant \def \Pr {\mathit {Pr}}\def \Fr {\mathit {Fr}}\def \Rey {\mathit {Re}}10^\circ $. It is shown that the energy transfer and the wavelength of the generated Brillouin peak depend on the plasma density, the intensity of the laser pulses, and the competition between two-plasmon decay and stimulated Raman scatter instabilities. The highest obtained energy transfer from pump to probe pulse is 2.5%, at a plasma density of $0.17 n_{cr}$, and this energy transfer increases significantly with plasma density. Therefore, our results suggest that much higher efficiencies can be obtained when higher densities (above $0.25 n_{cr}$) are used.

Copper activation was used to characterize high-energy proton beam acceleration from near-critical density plasma targets. An enhancement was observed when decreasing the target density, which is indicative for an increased laser-accelerated hot electron density at the rear target-vacuum boundary. This is due to channel formation and collimation of the hot electrons inside the target. Particle-in-cell simulations support the experimental observations and show the correlation between channel depth and longitudinal electric field strength is directly correlated with the proton acceleration.

We investigate the influence of the initial size of the proton layer on proton acceleration in the interaction of high intensity laser pulses with double-layer targets by using two-dimensional particle-in-cell code. We discuss the influence of proton layer initial sizes on the cut-off energy, energy spread, and divergence angle of proton beam. It is found that Coulomb explosion plays an important role on the proton cut-off energy. This causes the cut-off energy to increase for increasing proton layer thickness, at the expense of energy spread. The proton divergence angle reaches a peak value and then falls again with increasing the width. Proton divergence angle grows with target thickness. It is found that there is an optimal thickness to obtain the narrowest energy spread, which may provide an effective method (change the size of proton layer) to obtain high quality proton beams. This work may serve to improve the understanding of sheath field proton acceleration.

Self-modulated wakefield acceleration was investigated at densities down to ~4 × 1018 cm−3 by propagating the 50 TW 300 fs LULI laser in helium gas jets at lengths up to 1 cm. Long interaction lengths were achieved by closer matching of the initial focal spot size to the matched spot size for these densities. Electrons with energies extending to 180 MeV were observed in broad energy spectra which show some evidence for non-Maxwellian features at high energy. Two-dimensional PIC simulations indicate that the intial laser pulse breaks up into small pulselets that are eventually compressed and focused inside the first few plasma periods, leading to a ‘bubble-like’ acceleration of electron bunches.

As the state of the art for high power laser systems increases from terawatt to petawatt level and beyond, a crucial parameter for routinely monitoring high intensity performance is laser spot size on a solid target during an intense interaction in the tight focus regime (<10 µm). Here we present a novel, simple technique for characterizing the spatial profile of such a laser focal spot by imaging the interaction region in third harmonic order (3ωlaser). Nearly linear intensity dependence of 3ωlaser generation for interactions >1019 Wcm−2 is demonstrated experimentally and shown to provide the basis for an effective focus diagnostic. Importantly, this technique is also shown to allow in-situ diagnosis of focal spot quality achieved after reflection from a double plasma mirror setup for very intense high contrast interactions (>1020 Wcm−2) an important application for the field of high laser contrast interaction science.

A “table-top” high power laser has been used to generate beams of accelerated electrons up to energy of 20 MeV from interactions with underdense plasmas. The energy spectrum of these beams was measured using a magnetic spectrometer and proof-of-principle experiments were performed to evaluate the suitability of these beams for electron radiography applications.

Experiments were performed using high-power laser pulses (greater than 50 TW) focused into underdense helium, neon, or deuterium plasmas (ne ≤ 5 × 1019 cm−3). Ions having energies greater than 300 keV were measured to be produced primarily at 90° to the axis of laser propagation. Ion energies greater than 6 MeV were recorded from interactions with neon. Spatially resolved pinhole images of the ion emission were also obtained and were used to estimate the intensity of the focused radiation in the interaction region.

An experiment has been performed with the LULI Multi-TeraWatt Laser. The acceleration of electrons injected in a plasma wave generated by the laser wakefield mechanism has been observed with a maximum energy gain of 1.5 MeV. It has been shown that the electrons deflected during the interaction, could scatter on the walls of the experimental chamber, and fake a high-energy signal. A special effort has been given in the electron detection to separate the accelerated electrons signal from the background noise.The experimental results agree with theoretical predictions and numerical simulations when 3D effects on the electron beam are taken into account.

The frequency-doubling efficiency and resultant focal spot quality of a large aperture (140 × 89 mm) subpicosecond, chirped pulse amplified (CPA) 1054-nm beam for laser–matter interaction studies has been investigated using the Vulcan Nd:glass laser system (Danson et al. 1998). The effect of B-integral on the CPA beam quality was studied and is shown not to be the dominant cause of the observed frequency-doubled beam break-up. Conversion efficiency tests were carried out on small aperture KDP (type 1) crystals at a range of incident intensities up to 3 × 1011 W/cm2 giving the optimum crystal thickness for pulses in the 0.3–3 ps region. A large-aperture frequency-doubled beam was commissioned and delivered pulses of over 10 TW onto target for an electron acceleration experiment.

We report on multiphoton ionization experiments using picosecond (ps) and sub-ps UV-laser radiation at focused intensities up to 1018 W/cm2. The experiments are concerned with determining the electron temperature of optically ionized gases produced by intense KrF lasers. Thomson scattering, stimulated Raman scattering (SRS), and X-ray emission measurements have been made and compared with modeling calculations of heating. A particular objective is to identify the respective roles of above-threshold ionization, nonlinear inverse bremsstrahlung absorption, and SRS in determining the temperature of the electrons. Results for 350-fs pulses are compared with previous measurements for 12-ps pulses (for which strikingly different behavior is observed). The importance of using subps, short-wavelength lasers to minimize electron temperature is confirmed.