The post-compression technique based on self-phase modulation of high-energy pulses leads to an increase in achievable peak power and intensity. Typically, the pulses considered in experiments have been less than 100 fs in duration. Here, the method is applied to the ELFIE laser system at the LULI facility, for a pulse of 7 J energy and an initial measured duration of 350 fs. A 5-mm-thick fused silica window and a 2 mm cyclic-olefin polymer were used as optical nonlinear materials. The 9 cm diameter beam was spectrally broadened to a bandwidth corresponding to 124 fs Fourier-limited pulse duration, and then it was partly post-compressed to 200 fs. After measuring the spatial spectra of the beam fluence, a uniform gain factor of 4 increase in the fluctuations over the studied range of frequencies is observed, due to small-scale self-focusing.

Spectral-broadening of the APOLLON PW-class laser pulses using a thin-film compression technique within the long-focal-area interaction chamber of the APOLLON laser facility is reported, demonstrating the delivery of the full energy pulse to the target interaction area. The laser pulse at 7 J passing through large aperture, thin glass wafers is spectrally broadened to a bandwidth that is compatible with a 15-fs pulse, indicating also the possibility to achieve sub-10-fs pulses using 14 J. Placing the post-compressor near the interaction makes for an economical method to produce the shortest pulses by limiting the need for high damage, broadband optics close to the final target rather than throughout the entire laser transport system.

The objective of the Apollon 10 PW project is the generation of 10 PW peak power pulses of 15 fs at $1~\text{shot}~\text{min}^{-1}$. In this paper a brief update on the current status of the Apollon project is presented, followed by a more detailed presentation of our experimental and theoretical investigations of the temporal characteristics of the laser. More specifically the design considerations as well as the technological and physical limitations to achieve the intended pulse duration and contrast are discussed.

The objective of the Apollon project is the generation of 10 PW peak power pulses of 15 fs at 1 shot/minute. In this paper the Apollon facility design, the technological challenges and the current progress of the project will be presented.

The use of laser-accelerated protons as a particle probe for the detection of electric fields in plasmas has led in recent years to a wealth of novel information regarding the ultrafast plasma dynamics following high intensity laser-matter interactions. The high spatial quality and short duration of these beams have been essential to this purpose. We will discuss some of the most recent results obtained with this diagnostic at the Rutherford Appleton Laboratory (UK) and at LULI - Ecole Polytechnique (France), also applied to conditions of interest to conventional Inertial Confinement Fusion. In particular, the technique has been used to measure electric fields responsible for proton acceleration from solid targets irradiated with ps pulses, magnetic fields formed by ns pulse irradiation of solid targets, and electric fields associated with the ponderomotive channelling of ps laser pulses in under-dense plasmas.

The interaction of high-intensity laser pulses with matter releases instantaneously ultra-large currents of highly energetic electrons, leading to the generation of highly-transient, large-amplitude electric and magnetic fields. We report results of recent experiments in which such charge dynamics have been studied by using proton probing techniques able to provide maps of the electrostatic fields with high spatial and temporal resolution. The dynamics of ponderomotive channeling in underdense plasmas have been studied in this way, as also the processes of Debye sheath formation and MeV ion front expansion at the rear of laser-irradiated thin metallic foils. Laser-driven impulsive fields at the surface of solid targets can be applied for energy-selective ion beam focusing.

We present a novel technique for focusing and energy selection of high-current, MeV proton/ion beams. This method employs a hollow micro-cylinder that is irradiated at the outer wall by a high intensity, ultra-short laser pulse. The relativistic electrons produced are injected through the cylinder's wall, spread evenly on the inner wall surface of the cylinder, and initiate a hot plasma expansion. A transient radial electric field (107–1010 V/m) is associated with the expansion. The transient electrostatic field induces the focusing and the selection of a narrow band component out of the broadband poly-energetic energy spectrum of the protons generated from a separate laser irradiated thin foil target that are directed axially through the cylinder. The energy selection is tunable by changing the timing of the two laser pulses. Computer simulations carried out for similar parameters as used in the experiments explain the working of the micro-lens.

Due to their particular properties (low emittance, short duration, and large number density), the beams of multi-MeV protons generated during the interaction of ultraintense (I > 1019 W/cm2) short pulses with thin solid targets are suited for use as a particle probe in laser-plasma experiments. When traversing a sample, the proton density distribution is, in general, affected by collisional stopping, scattering and deflections via electromagnetic fields, and each of these effects can be used for diagnostic purposes. In particular, in the limit of very thin targets, the proton beams represent a valuable diagnostic tool for the detection of quasi-static electromagnetic fields. The proton imaging and deflectometry techniques employ these beams, in a point-projection imaging scheme, as an easily synchronizable diagnostic tool in laser- plasma interactions, with high temporal and spatial resolution. By providing diagnostic access to electro-magnetic field distributions in dense plasmas, this novel diagnostics opens up to investigation a whole new range of unexplored phenomena. Several transient processes were investigated employing this technique, via the detection of the associated electric fields. Examples provided in this paper include the detection of pressure-gradient electric field in extended plasmas, and the study of the electrostatic fields associated to the emission of MeV proton beams in high-intensity laser-foil interactions.

Since their discovery, laser accelerated ion beams have been the subject of great interest. The ion beam peak power and beam emittance is unmatched by any conventionally accelerated ion beam. Due to the unique quality, a wealth of applications has been proposed, and the first experiments confirmed their prospects. Laser ion acceleration is strongly linked to the generation and transport of hot electrons by the interaction of ultra-intense laser light with matter. Comparing ion acceleration experiments at laser systems with different beam parameters and using targets of varying thickness, material and temperature, some insight on the underlying physics can be obtained. The paper will present experimental results obtained at different laser systems, first beam quality measurement on laser accelerated heavy ions, and ion beam source size measurements at different laser parameters. Using structured targets, we compare information obtained from micro patterned ion beams about the accelerating electron sheath, and the influence of magnetic fields on the electron transport inside conducting targets.

The construction of short pulse (<200 fs) tunable X-ray laser sources based on the X-ray free electron laser (XFEL) concept will be a watershed for plasma-based and warm dense matter research. These new fourth generation light sources will have extremely high fields and short wavelengths (∼0.1 nm) with peak spectral brightnesses 1010 greater than third generation sources. Further, the high intensity upgrade of the GSI accelerator facilities will lead to specific energy depositions up to 200 kJ/g and temperatures between 1 and 10 eV at almost solid-state densities, enabling interesting experiments in the regime of nonideal plasmas, such as the evolution of intense ion beams in the interior of a Jovian planet. Below we discuss several applications: the creation of warm dense matter (WDM) research, probing of near solid density plasmas, and laser–plasma spectroscopy of ions in plasmas. The study of dense plasmas has been severely hampered by the fact that laser-based methods have been unavailable and these new fourth generation sources will remove these restrictions.

We use both a Fourier-transform-based analysis and time-retrieval calculations to get time-resolved measurements of the reflectivity and the phase shift of a chirped probe pulse interacting with a fs-laser-produced plasma by spectral interferometry in a single shot. We have devised a novel dual-quadrature Mach–Zehnder configuration in which wavefront division is used to obtain spatial fringes from the perturbed and unperturbed probe simultaneously. We demonstrate the capability of this technique with fully analyzed experimental data on the interaction of a femtosecond laser with C3H6 and C samples, showing 35-fs time resolution.

Electromagnetic emission at the plasma frequency ωp and its harmonics nωp has been studied. Although such emission is well known from very low density plasmas (electron density of the order of ne ≈ 108 cm−3) now, for the first time it has also been observed from a high density plasma (electron density of the order of ne ≈ 1023 cm−3) produced by a high-intensity femtosecond laser pulse. This radiation is strongly connected to jets of high energy electrons produced in such steep gradient plasmas by collective mechanisms, and probably to nonlinear Langmuir waves in the overdense plasma region. Theoretical investigations using particle-in-cell simulations have been made to pinpoint the physical origin and properties of the emission. Preliminary results show a very weak scaling of the ωp and 2ωp emission with intensity, which should provide clues for future theoretical analyses. Although not the main subject of the present work, also harmonics up to the 20th of the laser fundamental may have been observed close to the ωp and 2ωp line emission in the present experiment (PACS numbers: 52.40.Nk, 42.65.ky, 52.65.-y, 33.20.Ni, 52.25.Qt).

High intensity fs-laser pulses can deliver focused intensities in the region of 1016–1019 W/cm2. If the laser pulse is focused onto a solid or gaseous material, a plasma is created. The electrons, as well as the ions are accelerated in the strong laser field up to energies in the range of keV to several MeV. The interaction of the high energy particles with cold material, that is, the solid target yield of intense X-ray emission, K-shell—as well as bremsstrahlung-radiation. The K-shell emission from layered targets is a useful indicator of the production efficiency, energy distribution, and transport of hot electrons produced in fs-laser plasmas. For the diagnosis of laser plasma interaction and its application as an intense X-ray source, the spatial, temporal and spectral distribution of K-shell X rays is of fundamental importance. Focusing crystal spectrographs can be used to obtain a single shot X-ray spectra of laser plasmas produced by table top fs-lasers. With a spatial- and spectral-focusing spectrograph based on a toroidally bent crystal, the emission region of the hot plasma and Kα-radiation can be determined. Recording the spectra online by a frontside illuminated charge-coupled device (CCD) allows alignment of the crystal spectrograph, as well as the laser beam focusing leading to different X-ray source sizes. Using a controlled fs-prepulse, an increase in Kα radiation could be observed with the diagnostic.

Measurements of calibrated high resolution spectra are compared with particle-in-cell (PIC) calculations of the laser absorption and hot electron production postprocessed by a Monte–Carlo (MC) transport model of electron stopping and Kα X-ray generation.

Using the technique of frequency-domain interferometry, we demonstrate a new way of studying laser-induced breakdown at the surface of dielectric materials. A theoretical model based on electron production by multiphoton ionisation, inverse bremsstrahlung heating, and collisional ionisation is in quantitative agreement with both the detailed time variation of the dielectric constant and the pulse width variation of the fluence threshold. From the complex reflection coefficient measured with the two probe pulse polarisations in quadrature, we deduce the time variation of the dielectric constant of silica during breakdown.

The spectra of laser-produced plasmas of various materials of Z>70 have been interpreted as spin-orbit-split arrays of the 3d – 4f and 3d – 5f transitions for Ni-like to Ge-like ions. The excellent agreement between the model and the experiments indicated the possibility of their use for plasma diagnostics. First results from targets of Gold alloyed with Aluminium give an alternative diagnostic.

Spectral line profiles, broadened mostly by Stark effects from electric fields produced by charge particles, and diélectronic satellite line intensities have recently been used for determining electron densities in the dense region of laser-created plasmas. We present here a direct comparison of electron density measurements in the conduction region of laser created plasmas on a plane target using these two techniques.

Experiments were carried at the GRECO laser facility, using the Nd phosphate glass laser at its second harmonic (0.53 μm) and 600 ps pulse length. The laser was focused on a 160 μm focal spot in which was centered a 25 or 50 μm diameter aluminum dot implanted on a carbon substrate. Laser intensities were in the range 1 × 1014−3 × 1014 W/cm2. The ls4p−ls2 He-like transition, the 4p−ls H-like transition and the Ly c satellites were recorded on the same spectrum with a PET flat crystal spectrograph. Spot spectroscopy provided quasi-homogeneity and low reabsorption along the line of sight which was tilted 7° out the target surface. 3 μm resolution along the laser axis was obtained with an imaging knife-edge placed 1 mm apart from the target.

The dielectronic satellite lines from the ls21a 3lb and ls31a 31b, double-excited configurations of lithium-like ions have been studied experimentally and theoretically under dense-plasma conditions. Good agreement between theory and measurements performed in laser-target interactions at 0.53 m wavelength, 1014 W/cm2 laser irradiance show that collisional equilibrium conditions are reached between n − 3 singly and double excited levels at electron densities greater than 1022 cm−3 in Al and Si.