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Laboratory Radionuclide Migration Experiments at a Scale of 1 m

Published online by Cambridge University Press:  28 February 2011

Tjalle T. Vandergraaf
Affiliation:
Whiteshell Nuclear Research Establishment, Atomic Energy of Canada Limited, Pinawa, Manitoba ROE ILO Canada.
D. M. Grondin
Affiliation:
Whiteshell Nuclear Research Establishment, Atomic Energy of Canada Limited, Pinawa, Manitoba ROE ILO Canada.
D. J. Drew
Affiliation:
Whiteshell Nuclear Research Establishment, Atomic Energy of Canada Limited, Pinawa, Manitoba ROE ILO Canada.
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Abstract

Results are presented from a migration experiment carried out in a natural fracture in a 1 m × 1 m × 0.6 m quarried granite block. Near-uniform flow in the fracture was achieved by controlling the groundwater flow from the fracture laterally across the exit face of the fracture. The longitudinal dispersion was determined from the elution profile of uranine, a non-sorbing tracer. The effect of matrix diffusion was determined by reducing the linear velocity of the transport solution from approximately 3 to 0.75 cm/h. The velocity of a sorbing tracer, Cs-137, was compared to that of non-sorbing I-131 and with that calculated from data obtained for Cs-137 in static sorption experiments on similar fracture surfaces. Information on channeling in the fracture was obtained by autoradiographing the fracture surface of the separated block after the termination of the experiment. Quantitative information on the sorbed Cs-137 inventory by two-dimensional gamma scanning of the fracture surfaces is underway.

Type
Research Article
Copyright
Copyright © Materials Research Society 1988

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