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Enabling Solar Fuels Technology With High Throughput Experimentation

Published online by Cambridge University Press:  07 January 2014

J. M. Gregoire ,
J. A. Haber ,
S. Mitrovic ,
C. Xiang ,
S. Suram ,
P. F. Newhouse ,
E. Soedarmadji ,
M. Marcin ,
K. Kan  and
D. Guevarra
...Show all authors
J. M. Gregoire
Affiliation:
Joint Center for Artificial Photosynthesis, California Institute of Technology, Pasadena, California 91125, USA.
J. A. Haber
Affiliation:
Joint Center for Artificial Photosynthesis, California Institute of Technology, Pasadena, California 91125, USA.
S. Mitrovic
Affiliation:
Joint Center for Artificial Photosynthesis, California Institute of Technology, Pasadena, California 91125, USA.
C. Xiang
Affiliation:
Joint Center for Artificial Photosynthesis, California Institute of Technology, Pasadena, California 91125, USA.
S. Suram
Affiliation:
Joint Center for Artificial Photosynthesis, California Institute of Technology, Pasadena, California 91125, USA.
P. F. Newhouse
Affiliation:
Joint Center for Artificial Photosynthesis, California Institute of Technology, Pasadena, California 91125, USA.
E. Soedarmadji
Affiliation:
Joint Center for Artificial Photosynthesis, California Institute of Technology, Pasadena, California 91125, USA.
M. Marcin
Affiliation:
Joint Center for Artificial Photosynthesis, California Institute of Technology, Pasadena, California 91125, USA.
K. Kan
Affiliation:
Joint Center for Artificial Photosynthesis, California Institute of Technology, Pasadena, California 91125, USA.
D. Guevarra
Affiliation:
Joint Center for Artificial Photosynthesis, California Institute of Technology, Pasadena, California 91125, USA.
R. Jones
Affiliation:
Joint Center for Artificial Photosynthesis, California Institute of Technology, Pasadena, California 91125, USA.
N. Becerra
Affiliation:
Joint Center for Artificial Photosynthesis, California Institute of Technology, Pasadena, California 91125, USA.
E. W. Cornell
Affiliation:
Engineering Division and Joint Center for Artificial Photosynthesis, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA.
J. Jin
Affiliation:
Engineering Division and Joint Center for Artificial Photosynthesis, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA.
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Abstract

The High Throughput Experimentation (HTE) project of the Joint Center for Artificial Photosynthesis (JCAP, http://solarfuelshub.org/) performs accelerated discovery of new earth-abundant photoabsorbers and electrocatalysts. Through collaboration within the DOE solar fuels hub and with the broader research community, the new materials will be utilized in devices that efficiently convert solar energy, water and carbon dioxide into transportation fuels. JCAP-HTE builds high-throughput pipelines for the synthesis, screening and characterization of photoelectrochemical materials. In addition to a summary of these pipelines, we will describe several new screening instruments for high throughput (photo-)electrochemical measurements. These instruments are not only optimized for screening against solar fuels requirements, but also provide new tools for the broader combinatorial materials science community. We will also describe the high throughput discovery, follow-on verification, and device implementation of a new quaternary metal oxide catalyst. This rapid technology development from discovery to device implementation is a hallmark of the multi-faceted JCAP research effort.

Keywords

combinatorial synthesisphotochemicalenergy generation
Type
Articles
Information
MRS Online Proceedings Library (OPL) , Volume 1654: Symposium NN – Adaptive Soft Matter through Molecular Networks , 2014 , mrsf13-1654-nn07-02
Copyright
Copyright © Materials Research Society 2014 

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References

REFERENCES

Pinaud, B. A.; Benck, J. D.; Seitz, L. C.; Forman, A. J.; Chen, Z. B.; Deutsch, T. G.; James, B. D.; Baum, K. N.; Baum, G. N.; Ardo, S.; Wang, H. L.; Miller, E.; Jaramillo, T. F., Technical and economic feasibility of centralized facilities for solar hydrogen production via photocatalysis and photoelectrochemistry. Energy & Environmental Science 2013, 6, (7), 1983–2002.CrossRefGoogle Scholar
Walter, M. G.; Warren, E. L.; McKone, J. R.; Boettcher, S. W.; Mi, Q. X.; Santori, E. A.; Lewis, N. S., Solar Water Splitting Cells. Chemical Reviews 2010, 110, (11), 6446–6473.CrossRefGoogle ScholarPubMed
Bard, A. J.; Fox, M. A., Artificial Photosynthesis - Solar Splitting of Water to Hydrogen and Oxygen. Accounts of Chemical Research 1995, 28, (3), 141–145.CrossRefGoogle Scholar
Haussener, S.; Xiang, C. X.; Spurgeon, J. M.; Ardo, S.; Lewis, N. S.; Weber, A. Z., Modeling, simulation, and design criteria for photoelectrochemical water-splitting systems. Energy & Environmental Science 2012, 5, (12), 9922–9935.CrossRefGoogle Scholar
Basic research needs for solar energy utilization; U.S. Department of Energy (DOE), Office of Basic Energy Sciences,: Washington, D.C., 2005.Google Scholar
Lewis, N. S., Toward cost-effective solar energy use. Science 2007, 315, (5813), 798–801.CrossRefGoogle ScholarPubMed
Calvert, P., Inkjet printing for materials and devices. Chemistry of Materials 2001, 13, (10), 3299–3305.CrossRefGoogle Scholar
Liu, X. N.; Shen, Y.; Yang, R. T.; Zou, S. H.; Ji, X. L.; Shi, L.; Zhang, Y. C.; Liu, D. Y.; Xiao, L. P.; Zheng, X. M.; Li, S.; Fan, J.; Stucky, G. D., Inkjet Printing Assisted Synthesis of Multicomponent Mesoporous Metal Oxides for Ultrafast Catalyst Exploration. Nano Letters 2012, 12, (11), 5733–5739.CrossRefGoogle ScholarPubMed
Gregoire, J. M.; Xiang, C.; Mitrovic, S.; Liu, X.; Marcin, M.; Cornell, E. W.; Fan, J.; Jin, J., Combined Catalysis and Optical Screening for High Throughput Discovery of Solar Fuels Catalysts. Journal of the Electrochemical Society 2013, 160, (4), F337–F342.CrossRefGoogle Scholar
Gregoire, J. M.; Xiang, C. X.; Liu, X. N.; Marcin, M.; Jin, J., Scanning droplet cell for high throughput electrochemical and photoelectrochemical measurements. Review of Scientific Instruments 2013, 84, (2).Google ScholarPubMed