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Dynamic Control of Plasmon-Exciton Coupling in Au Nanodisk–J-Aggregate Hybrid Nanostructure Arrays

Published online by Cambridge University Press:  31 January 2011

Yue Bing Zheng ,
Bala Krishna Juluri ,
Linlin Jensen ,
Lasse Jensen  and
Tony Jun Huang
Yue Bing Zheng
Affiliation:
yzz113@psu.edu, The Pennsylvania State University, Department of Engineering Science and Mechanics, University Park, Pennsylvania, United States
Bala Krishna Juluri
Affiliation:
juluribk@gmail.com
Linlin Jensen
Affiliation:
luz11@psu.edu, The Pennsylvania State University, Department of Chemistry, University Park, Pennsylvania, United States
Lasse Jensen
Affiliation:
jensen@chem.psu.edu, The Pennsylvania State University, Department of Chemistry, University Park, Pennsylvania, United States
Tony Jun Huang
Affiliation:
junhuang@psu.edu, The Pennsylvania State University, Department of Engineering Science and Mechanics, University Park, Pennsylvania, United States
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Abstract

We report the dynamic control of plasmon-exciton coupling in Au nanodisk arrays adsorbed with J-aggregate molecules by incident angle of light. The angle-resolved spectra of an array of bare Au nanodisks exhibit continuous shifting of localized surface plasmon resonances. This characteristic enables the production of real-time, controllable spectral overlaps between molecular and plasmonic resonances, and the efficient measurement of plasmon-exciton coupling as a function of wavelength with one or fewer nanodisk arrays. Experimental observations of varying plasmon-exciton coupling match with coupled dipole approximation calculations.

Keywords

optical propertiesmetalnanostructure
Type
Research Article
Information
MRS Online Proceedings Library (OPL) , Volume 1208: Symposium O – Excitons and Plasmon Resonances in Nanostructures II , 2009 , 1208-O15-02
Copyright
Copyright © Materials Research Society 2010

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