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Environmental Isotope Study (14C, 13C, 18O, D, Noble Gases) on Deep Groundwater Circulation Systems in Hungary With Reference to Paleoclimate

Published online by Cambridge University Press:  18 July 2016

Martin Stute
Affiliation:
Institute of Environmental Physics, Im Neuenheimer Feld 366 D-6900 Heidelberg, FRG
Jozsef Deak
Affiliation:
Institute of Environmental Physics, Im Neuenheimer Feld 366 D-6900 Heidelberg, FRG
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Abstract

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We have studied environmental isotopes and noble gases in groundwater samples from various locations in the Great Hungarian Plain along two selected hydrogeological cross-sections of ca 100km. The 14C groundwater ages were corrected hydrochemically and compared with age information derived from excess helium due to 4He from α-decay of U and Th and their daughter nuclides within the aquifer and to He accumulation from the crustal (and mantle) He flux. In correcting the 14C groundwater ages, we considered carbonate dissolution under open and closed system conditions in the infiltration areas. Non-radioactive reduction of the 14C/12C isotope ratio also plays an important role due to the addition of “dead” carbon species to groundwater along its subsurface pathway. High (corrected) 14C ages, which fall into the last global cold period, are supported by significantly lower heavy stable isotope values as well as lower temperatures derived from the noble gases Ne, Ar, Kr and Xe.

Type
IV. Applications
Copyright
Copyright © The American Journal of Science 

References

Deák, J, Stute, M, Rudolph, J and Sonntag, C, 1987, Determination of the flow regime of Quaternary and Pliocene layers in the Great Hungarian Plain (Hungary) by D, 18O, 14C and noble gas measurements, in Isotope techniques in water resources development: IAEA, Vienna, p 335350.Google Scholar
Deines, P, Langmuir, D and Harmon, R S, 1974, Stable carbon isotope ratio and the existence of a gas phase in the evolution of carbonate groundwaters: Geochim et Cosmochim Acta, v 38, p 11471164.CrossRefGoogle Scholar
Dörr, H and Münnich, K O, 1987, Annual variation in soil respiration in selected areas on the temperate zone: Tellus, v 39B, p 114121.Google Scholar
Dörr, H, Sonntag, C and Regenberg, W, 1987, Field study of the initial 14C content as a limiting factor in 14C groundwater dating, in Isotope techniques in water resources development: IAEA, Vienna, p 7386.Google Scholar
Erdélyi, M, 1976, Outlines of the hydrodynamics and hydrochemistry of the Pannonian Basin: Acta Geol Acad Sci Hungaricae, v 20, no. 3–4, p 287309.Google Scholar
Frenzel, B, 1980, Klima der letzten Eiszeit und der Nacheiszeit in Europa: Veröffentlichungen Joachim Jungius-Gesell Wiss, Hamburg, v 44, p 946.Google Scholar
Fritz, P and Fontes, J Ch, eds, 1980, Handbook of environmental isotope geochemistry I: Amsterdam, Elsevier, p 4974.Google Scholar
Garrels, R M and Christ, C L, 1965, Solutions, minerals and equilibra: New York, Harper & Row.Google Scholar
Heaton, T H E and Vogel, J C, 1981, “Excess air” in groundwater: Jour Hydrology, v 50, p 201216.CrossRefGoogle Scholar
Jähne, B, Heinz, G and Dietrich, W, 1987, Measurement of the diffusion coefficients of sparingly soluble gases in water: Jour Geophys Research, v 92, no. C10, p 1076710776.CrossRefGoogle Scholar
Mamyrin, B A and Tolstikhin, I N, 1984, Helium isotopes in nature, in Developments in geochemistry 3: Amsterdam, Elsevier, p 210.Google Scholar
Mazor, E, 1972, Paleotemperatures and other hydrological parameters deducted from noble gases dissolved in groundwaters, Jordan Rift Valley Israel: Geochim et Cosmochim Acta, v 36, p 13211336.Google Scholar
Pearson, F J Jr, 1965, Use of 13C/12C ratios to correct radiocarbon ages of materials initially diluted by limestones, in Chatters, R M and Olson, E A, eds, Internatl conf on 14C & tritium dating, 6th, Proc: Clearinghouse Fed Sci Tech Inf, NBS, Washington, DC, p 357366.Google Scholar
Pearson, F J Jr and Swarzenki, W V, 1974, 14C evidence for the origin of arid region groundwater, Northeastern Providence, Kenya, in Isotopes in groundwater hydrology, 2: IAEA, Vienna, p 95108.Google Scholar
Rudolph, J, Rath, H K and Sonntag, C, 1984, Noble gases and stable isotopes in 14C-dated paleowaters from central Europe and the Sahara, in Isotope hydrology: IAEA, Vienna, p 467477.Google Scholar
Torgersen, T and Ivey, G N, 1985, Helium accumulation in groundwater II: A model for the accumulation of the crustal 4He degassing flux: Geochim et Cosmochim Acta, v 49, p 24452452.Google Scholar