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Nanoscale investigation of polar structure of (1-x)PbMg1/3Nb2/3O3-xPbTiO3 single crystals

  • V. V. Shvartsman (a1), M. Wojtas (a2), S. Vakhrushev (a3) and A. L. Kholkin (a1)

Abstract

ABSTRACT (1-x)PbMg1/3Nb2/3O3-xPbTiO3 (PMN-PT) single crystals of different compositions were studied via piezoresponse force microscopy (PFM). Piezoelectric contrast has been observed in 0.9PMN-0.1PT above the temperature of structural transition indicating spatial distribution of polarization and was attributed to the existence of polar clusters. The domain patterns were found to change drastically with increasing Ti content. In particular, the piezoresponse images of 0.8PMN-0.2PT combine both relaxor and ferroelectric features and in 0.65PMN-0.35PT crystals only micron-sized ferroelectric domains were observed. The evolution of the polar structures with increasing temperature and under external electric field was also investigated. The nature of the observed phenomena is discussed based on the current understanding of the relaxor state in ferroelectrics and possible influence of PFM instrumentation

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1. Park, S.-E., Shrout, T. R., J. Appl. Phys., 82, 1804 (1997).10.1063/1.365983
2. Vakhrushev, S., Naberezhnov, A., Sinha, S. K., Feng, Y. P., and Egami, T., J. Phys. Chem. Solids, 57, 1517 (1996).10.1016/0022-3697(96)00022-4
3. Vakhrushev, S. B., Kvyatkovsky, B. E., Naberezhnov, A. A., Okuneva, N. M., and Toperverg, B. P., Ferroelectrics, 90, 173 (1989).10.1080/00150198908211287
4. Miao, S., Zhu, J., Zhang, X., and Cheng, Z.-Y., Phys. Rev. B, 65, 052101 (2001).10.1103/PhysRevB.65.052101
5. Gruverman, A., Auciello, O., and Tokumoto, H., Annu. Rev. Mater. Sci. 28, 101 (1998).10.1146/annurev.matsci.28.1.101
6. Smolenskii, G. A., Isupov, V. A., Agranovskaja, A. I., and Popov, S. N., Sov. Phys. Solid State 2, 2584 (1960).
7. de Mathant, N., Hussont, E., Calvarint, G., Gavarris, J. R., Hewat, A. W., and Morell, A, J. Phys.: Condens. Matter. 3, 8159 (1991).
8. Noblanc, O., Gaucher, P., and Calvarin, G., J. Appl. Phys. 79, 4261 (1996).10.1063/1.361865
9. Dkhil, B., Kiat, J. M., Calvarin, G., Baldinozzi, G., Vakhrushev, S. B., and Suard, E., Phys. Rev. B 65, 024104 (2002).10.1103/PhysRevB.65.024104
10. Ye, Z.-G., Bing, Y., Gao, J., Bokov, A. A., Stephens, P., Noheda, B., and Shirane, G., Phys. Rev. B 67, 104104 (2003).10.1103/PhysRevB.67.104104
11. Xu, G., Viehland, D., Li, J. F., Gehring, P. M., and Shirane, G., cond-mat/0307144 v2 (unpublished).
12. Munoz, R. C., Vidal, G., Mulsow, M., Lisoni, J. G., Arenas, C., and Concha, A., Phys. Rev. B, 62, 4686 (2000).10.1103/PhysRevB.62.4686
13. Vakhrushev, S. B., Naberezhnov, A. A., Dkhil, B., Kiat, J.-M., Shvartsman, V., Kholkin, A., Dorner, B., and Ivanov, A., AIP Conf. Proc. 67, 74 (2003).10.1063/1.1609940
14. Lehnen, P., Kleemann, W., Woike, Th., Pankrath, P., Phys. Rev. B 64, 224109 (2001).10.1103/PhysRevB.64.224109
15. Bdikin, I. K., Shvartsman, V. V., and Kholkin, A. L., Appl. Phys. Lett. 83, 4232 (2003).10.1063/1.1627476
16. Samara, G. A., J. Phys.: Condens. Matter 15, R367 (2003).
17. Xu, G., Shirane, G., Copley, J. R. D., and Gehring, P. M., cond-mat/0308170 v2 (unpublished).
18. Noheda, B., Cox, D. E., Shirane, G., Gao, J., and Ye, Z.-G., Phys. Rev. B 66, 054104 (2002).10.1103/PhysRevB.66.054104
19. Bokov, A. A. and Ye, Z.-G., J. Appl. Phys. 91, 6656 (2002)10.1063/1.1471371

Nanoscale investigation of polar structure of (1-x)PbMg1/3Nb2/3O3-xPbTiO3 single crystals

  • V. V. Shvartsman (a1), M. Wojtas (a2), S. Vakhrushev (a3) and A. L. Kholkin (a1)

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