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Growth Evolution of (Zn,Cd)Se Quantum Dots Deduced from Spatially Resolved Structural and Optical Characterization

Published online by Cambridge University Press:  10 February 2011

K. Leonard
Affiliation:
Institute of Solid State Physics, University of Bremen, Germany
D. Hommel
Affiliation:
Institute of Solid State Physics, University of Bremen, Germany
A. Stockmann
Affiliation:
Institute of Materials Physics and Structural Research, University of Bremen, Germany
H. Selke
Affiliation:
Institute of Materials Physics and Structural Research, University of Bremen, Germany
J. Seufert
Affiliation:
Technical Physics, University of Wtirzburg, Germany
R. Weigand
Affiliation:
Technical Physics, University of Wtirzburg, Germany
G. Bacher
Affiliation:
Technical Physics, University of Wtirzburg, Germany
A. Forchel
Affiliation:
Technical Physics, University of Wtirzburg, Germany
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Abstract

The growth mode of CdSe layers grown by migration enhanced epitaxy between ZnSe barriers has been investigated. In situ reflection high-energy electron diffraction shows a gradual transition to a three-dimensional growth mode which, however, is not accompanied by a change of the surface lattice constant. High-resolution transmission electron micrographs reveal a strong Cd diffusion, leading to ternary ZnCdSe quantum wells. Furthermore. composition fluctuations perpendicular to the growth direction on a nanometer scale are found already prior to the beginning of the growth mode transition. In the case of heterostructures containing a CdSe layer that has undergone the growth mode transition, micrographs show Cd-rich quantum dots with diameters of around 8 nm and heights of around 1.5 nm within a ternary quantum well. By spatially resolved photoluminescence the emission from single quantum dots could be observed. The polarization dependence of the emission from single dots indicates an asymmetric shape of the dots with certain preferential orientations along the [110] and [110] directions.

Type
Research Article
Copyright
Copyright © Materials Research Society 2000

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References

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