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Exact Optical Susceptibilities of Three State Systems Interacting with a Single Frequency Electric Field
Published online by Cambridge University Press: 25 February 2011
Abstract
Using Floquet theory together with density matrix formalism, an exact, nonpertur-bative expression for the optical susceptibility of a three level system interacting with a single mode electric field is derived. By using a three state model that mimics a polymeric system, it is shown that in certain cases, using typical values for the intensity of the electric field, successive terms in the series χω=χ(1) + χ(3) E2… approach the same of order magnitude.
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- Copyright © Materials Research Society 1992