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Time-domain Brillouin Scattering as a Local Temperature Probe in Liquids

Published online by Cambridge University Press:  02 January 2019

Ievgeniia Chaban
Affiliation:
Institut des Molécules et Matériaux du Mans, UMR CNRS 6283, Le Mans Université, 72085 Le Mans, France Laboratoire d’Acoustique de l’Université du Maine, UMR CNRS 6613, Le Mans Université, 72085 Le Mans, France
Hyun D. Shin
Affiliation:
Department of Chemistry, Massachusetts Institute of Technology, Cambridge, MA 02139, USA
Christoph Klieber
Affiliation:
Department of Chemistry, Massachusetts Institute of Technology, Cambridge, MA 02139, USA
Rémi Busselez
Affiliation:
Institut des Molécules et Matériaux du Mans, UMR CNRS 6283, Le Mans Université, 72085 Le Mans, France
Vitaly Gusev
Affiliation:
Laboratoire d’Acoustique de l’Université du Maine, UMR CNRS 6613, Le Mans Université, 72085 Le Mans, France
Keith Nelson
Affiliation:
Department of Chemistry, Massachusetts Institute of Technology, Cambridge, MA 02139, USA
Thomas Pezeril
Affiliation:
Institut des Molécules et Matériaux du Mans, UMR CNRS 6283, Le Mans Université, 72085 Le Mans, France
Corresponding
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Abstract

We present results of time-domain Brillouin scattering (TDBS) to determine the local temperature of liquids. TDBS is based on an ultrafast pump-probe technique to determine the light scattering frequency shift caused by the propagation of coherent acoustic waves in a sample. Since the temperature influences the Brillouin scattering frequency shift, the TDBS signal probes the local temperature of the liquid. Results for the extracted Brillouin scattering frequencies recorded at different liquid temperatures and at different laser powers are shown to demonstrate the usefulness of TDBS as a temperature probe.

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Copyright
Copyright © Materials Research Society 2018 

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