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Direct Observation of Electrolyte Degradation Mechanisms in Li-Ion Batteries

  • B. Layla Mehdi (a1), Patricia Abellan (a1), Lucas R. Parent (a1), Meng Gu (a2), Chiwoo Park (a3), Wu Xu (a4), Yaohui Zhang (a4) (a5), Ilke Arslan (a4), Ji-Guang Zhang (a4), Chong-Min Wang (a2), James E. Evans (a2) and Nigel D. Browning (a1)...
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Abstract

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References

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[1] Xu, K., Chem, K. Rev., 104 (2004), p. 4303.
[2] Nasybulin, E., Xu, W., Engelhard, M. H., Nie, Z. M., Burton, S. D., Cosimbescu, L., Gross, M. E., Zhang, J. G. J Phys Chem C, 117 (2013), p. 2635.
[3] Verma, P., Maire, P., Novak, P. Electrochim Acta 55 (2010), p. 6332.
[4] The research described in this paper is part of the Chemical Imaging Initiative; it was conducted under the Laboratory Directed Research and Development Program at PNNL, a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. The electrolytes used in this work were prepared with the support from Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. Development of in-situ stages was supported by DOE NNSA-SSAA grant number DE-FG52-06NA26213, and DOE BES grant number DE-FG02-03ER46057. C.P. acknowledges support from the FSU COFRS Award 032968, the Ralph E. Powe Junior Faculty Enhancement Award, and NSF-CMMI-1334012.

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