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Radiation Effects in Glasses Used for Immobilization of High-level Waste and Plutonium Disposition

  • William J. Weber (a1), Rodney C. Ewing (a2), C. Austen Angell (a3), George W. Arnold (a4), Alastair N. Cormack (a5), Jean Marc Delaye (a6), David L. Griscom (a7), Linn W. Hobbs (a8), Alexandra Navrotsky (a9), David L. Price (a10), A. Marshall Stoneham (a11) and Michael C. Weinberg (a12)...

Abstract

This paper is a comprehensive review of the state-of-knowledge in the field of radiation effects in glasses that are to be used for the immobilization of high-level nuclear waste and plutonium disposition. The current status and issues in the area of radiation damage processes, defect generation, microstructure development, theoretical methods and experimental methods are reviewed. Questions of fundamental and technological interest that offer opportunities for research are identified.

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1.Closing the Circle on the Splitting of the Atom (U.S. Department of Energy, Office of Environmental Management, Washington, DC, 1995).
2.Management and Disposition of Excess Weapons Plutonium (National Academy Press, Washington, DC, 1994).
3.Management and Disposition of Excess Weapons Plutonium–Reactor-Related Options (National Academy Press, Washington, DC, 1995).
4.Wicks, G. G., Lodding, A. R., and Molecke, M. A., MRS Bull. XVIII (9), 33 (1993).
5.Jantzen, C. M., J. Am. Ceram. Soc. 75 (9), 2433 (1992).
6.Grambow, B., MRS Bull. XIX (12), 20 (1994).
7.Storage and Disposition of Weapons-Usable Fissile Materials Draft Programmatic Environmental Impact Statement, DOE/EIS-0229-D (U.S. Department of Energy, Washington, DC, 1996).
8.Defense Waste Processing Facility - Cost, Schedule, and Technical Issues, GAO/RCED 92-183 (U.S. General Accounting Office, Washington, DC, 1992).
9.Lutze, W., presented at the National Research Council Workshop on Glass as a Waste Form and Vitrification Technology, Washington, DC, May 13–15, 1996 (unpublished).
10.Cunnane, and Allison, J. M., in Scientific Basis for Nuclear Waste Management XVII, edited by Barkatt, A. and R. A. Van, Konynenburg (Mater. Res. Soc. Symp. Proc. 333, Pittsburgh, PA, 1994), p. 3.
11.Waste Form Compliance Plan for the West Valley Demonstration Project High-Level Waste Form, WVDP-185 (West Valley Demonstration Project, West Valley, NY, 1995).
12.Amerine, D. B., presented at the National Research Council Workshop on Glass as a Waste Form and Vitrification Technology, Washington, DC, May 13–15, 1996 (unpublished).
13.Illman, D. L., Chemical & Engineering News 71 (25), 9 (1993).
14. Office of Technology Assessment, Complex Cleanup: The Environmental Legacy of Nuclear Weapons Production, OTA-O-484 (Congress of the United States, Washington, DC, 1991).
15.Disposal of Weapon Plutonium, edited by Merz, E. R. and Walter, C. E. (Kluwer Academic Publishers, The Netherlands, 1996).
16.Makhijani, A. and Makhijani, A., Fissile Materials in a Glass, Darkly (IEER Press, Takoma Park, MD, 1995).
17.Browne, E., Dairiki, J. M., and Doebler, R. E., Table of Isotopes, edited by Lederer, C. M. and Sherley, V. S., 7th ed. (John Wiley and Sons, New York, 1978).
18.Taubes, G., Science 268, 1836 (1995).
19.Bowman, C. D. and Venneri, F., Sci. Glob. Secur. 5, 279 (1996).
20.Van Konynenburg, R. A., Sci. Glob. Secur. 5, 303 (1996).
21.Bibler, N. E., Ramsey, W. G., Meaker, T. F., and Pareizs, J. M., in Scientific Basis for Nuclear Waste Management XIX, edited by Murphy, W. M. and Knecht, D. A. (Mater. Res. Soc. Symp. Proc. 412, Pittsburgh, PA, 1996), p. 65.
22.Bates, J. K., Ellison, A. J. G., Emery, J. W., and Hoh, J. C., in Scientific Basis for Nuclear Waste Management XIX, edited by Murphy, W. M. and Knecht, D. A. (Mater. Res. Soc. Symp. Proc. 412, Pittsburgh, PA, 1996), p. 57.
23.Matzke, Hj., Special issue for a workshop on Radiation Damage Effects in Nuclear Waste Materials, Nucl. Instrum. Methods in Phys. Res. B 32, 453 (1988).
24.Weber, W. J., Mansur, L. K., Clinard, F. W., Jr., and Parkin, D. M., J. Nucl. Mater. 184, 1 (1991).
25.Weber, W. J. and Roberts, F. P., Nucl. Technol. 60, 178 (1983).
26.Burns, W. G., Hughes, A. E., Marples, J. A. C., Nelson, R. S., and Stoneham, A. M., J. Nucl. Mater. 107, 245 (1982).
27.Burns, W. G., Hughes, A. E., Marples, J. A. C., Nelson, R. S., and Stoneham, A. M., in Scientific Basis for Nuclear Waste Management V, edited by Lutze, W. (Mater. Res. Soc. Symp. Proc. 11, Pittsburgh, PA, 1982), p. 339.
28.Day, D. H., Hughes, A. E., Leake, J. W., Marples, J. A. C., Marsh, G. P., Rae, J., and Wade, B. O., Rep. Prog. Phys. 48, 101 (1985).
29.Weber, W. J., Nucl. Instrum. Methods in Phys. Res. B 32, 471 (1988).
30.Weber, W. J., J. Minerals, Metals and Materials Sociery 43 (7), 35 (1991).
31.Wronkiewicz, D. J., Effects of Radionuclide Decay on Waste Glass Behavior–A Critical Review, ANL-93/45 (Argonne National Laboratory, Argonne, IL, 1993).
32.Ewing, R. C., Weber, W. J., and Clinard, F. W., Jr., Progress in Nuclear Energy 29 (2), 63 (1995).
33.Weber, W. J. and Ewing, R. C., in Scientific Basis for Nuclear Waste Management XVIII, edited by Murakami, T. and Ewing, R. C. (Mater. Res. Soc. Symp. Proc. 353, Pittsburgh, PA, 1995), p. 1389.
34.Weber, W. J., Ewing, R. C., and Lutze, W., in Scientific Basis for Nuclear Waste Management XIX, edited by Murphy, W. M. and Knecht, D. A. (Mater. Res. Soc. Symp. Proc. 412, Pittsburgh, PA, 1996), p. 25.
35.Radioactive Waste Forms for the Future, edited by Lutze, W. and Ewing, R. C. (North-Holland, Amsterdam, 1988).
36.Ewing, R. C., J. Nucl. Mater. 190, vii (1992).
37.Buscheck, T. A., Nitao, J. J., and Ramspott, L. D., in Scientific Basis for Nuclear Waste Management XIX, edited by Murphy, W. M. and Knecht, D. A. (Mater. Res. Soc. Symp. Proc. 412, Pittsburgh, PA, 1996), p. 715.
38.Ziegler, J. F., Biersack, J. P., and Littmark, U., The Stopping and Range of Ions in Solids (Pergamon, New York, 1985).
39.Gray, W. J., Nature (London) 296, 547 (1982).
40.Turcotte, R. P., Radiation Effects in Solidified High-Level Wastes–Part 2, Helium Behavior, BNWL-2051 (Pacific Northwest National Laboratory, Richland, WA, 1976).
41.Sato, S., Furuya, H., Morikawa, K., Sugisaki, M., and Inagaki, Y., J. Nucl. Sci. and Technol. 27, 343 (1990).
42.Todd, B. J., Lineweaver, J. L., and Kerr, J. T., J. Appl. Phys. 31, 51 (1960).
43.Lineweaver, J. L., J. Appl. Phys. 34, 1786 (1963).
44.Bibler, N. E., in Scientific Basis for Nuclear Waste Management, edited by Topp, S. V. (Mater. Res. Soc. Symp. Proc. 6, North-Holland, New York, 1982), p. 681.
45.Standard Method for Testing the Long Term Alpha Irradiation Stability of Solidified High-Level Radioactive Waste Forms, ISO 6962 (International Organization for Standardization, Geneva, Switzerland, 1982).
46.Nuclear Waste Materials Handbook, Test Methods, DOE/TIC-11400 (Pacific Northwest Laboratory, Richland, WA, 1981).
47.Weber, W. J., Wald, J. W., and McVay, G. L., J. Am. Ceram. Soc. 68 (9), C-253 (1985).
48.Wagner, G. and van den Haute, P., Fission-Track Dating (Kluwer Academic Publishers, Dordrecht, The Netherlands, 1992).
49.Eyal, Y. and Ewing, R. C., in Proceedings of the International Conference on Nuclear Waste Management and Environmental Remediation, Vol. 1, edited by Alexandre, D., Baker, R., Kohout, R., and Marek, J. (ASME Press, New York, 1993), p. 191.
50.Fleischer, R. L., Science, 207, 979 (1980).
51.Arnold, G. W., Northrup, C. J. M., and Bibler, N. E., in Scientific Basis for Nuclear Waste Management-V, edited by Lutze, W. (Mater. Res. Soc. Symp. Proc. 11, Pittsburgh, PA, 1982), p. 357.
52.Malow, G. and Andresen, H., in Scientific Basis for Nuclear Waste Management, Vol. 1, edited by McCarthy, G. J. (Plenum Press, New York, 1979), p.109.
53.Antonini, M., Lanza, F., and Manara, A., in Ceramics in Nuclear Waste Management, edited by Chikalla, T. D. and Mendel, J. E., CONF-790420 (National Technical Information Service, Springfield, VA, 1979), p. 289.
54.Curtiss, L. F., Nature (London) 120, 406 (1927).
55.Lind, S. C., Science 68, 643 (1928).
56.Tuck, D. G., Int. J. Appl. Radiat. Isotopes 15, 49 (1964).
57.Lell, E., Kreidl, N. J., and Hensler, J. R., in Progress in Ceramic Science, Vol. 4, edited by Burke, J. (Pergamon Press, Oxford, New York, 1966), p. 1.
58.Griscom, D. L., in Glass: Science and Technology Vol. 4B, edited by Uhlmann, D. R. and Kreidl, N. J. (Academic Press, Boston, 1990), p. 151.
59.Clinard, F. W. Jr and Hobbs, L. W., in Physics of Radiation Effects in Crystals, edited by Johnson, R. A. and Orlov, A. N. (Elsevier, Amsterdam, 1986), p. 387.
60.Devine, R. A. B., Nucl. Instrum. Methods in Phys. Res. B 91, 378 (1994).
61.Farges, F., Ewing, R. C., and Brown, G. E., Jr., J. Mater. Res. 8, 1983 (1993).
62.Hobbs, L. W., J. Non-Cryst. Solids 192 & 193, 79 (1995).
63.Wright, A. C., Bachra, B., Brunier, T. M., Sinclair, R. N., Gladden, L. F., and Portsmouth, R. L., J. Non-Cryst. Solids 150, 69 (1992).
64.Hobbs, L. W., Nucl. Instrum. Methods in Phys. Res. B 91, 3042 (1994).
65.Marians, C. S. and Hobbs, L. W., J. Non-Cryst. Solids 119, 269 (1990).
66.Gladden, L. F., J. Non-Cryst. Solids 119, 318 (1990).
67.Vashishta, P., Nakano, A., Kalia, R. K., and Ebbsjo, I., J. Non-Cryst. Solids 182, 59 (1995).
68.Revesz, A. G. and Gibbs, G. V., in The Physics of MOS Insulators, edited by Lucovsky, G., Pantelides, S. T., and Galeener, F. L. (Pergamon, New York, 1980), p. 92.
69.Marians, C. S. and Burdett, J. K., J. Non-Cryst. Solids 124, 1 (1990).
70.Friebele, E. J., Griscom, D. L., Stapelbroek, M., and Weeks, R. A., Phys. Rev. Lett. 42, 1346 (1979).
71.Hobbs, L. W. and Pascucci, M. R., J. Phys. 41 (C6), 237 (1980).
72.Wooten, F. and Weaire, D., J. Non-Cryst. Solids 64, 325 (1984).
73.Jain, U., Powell, A. C., and Hobbs, L. W., in Defects in Materials, edited by Bristowe, P. D., Epperson, J. E., Griffith, J. E., and Z., Lillental-Weber (Mater. Res. Soc. Symp. Proc. 209, Pittsburgh, PA, 1991), p. 201.
74.Jacobs, D. J. and Thorpe, M. F., Phys. Rev. E 52, 3682 (1996).
75.Gupta, P. K., J. Am. Ceram. Soc. 76, 1088 (1993).
76.Greaves, G. N., J. Non-Cryst. Solids 71, 203 (1985).
77.Sales, B. C., Ramey, J. O., McCallum, J. C., and Boatner, L. A., J. Non-Cryst. Solids 126, 179 (1990).
78.Primak, W., Fuchs, L. H., and Day, P., Phys. Rev. 92, 1064 (1953).
79.Primak, W., Phys. Rev. 110, 1240 (1958).
80.Whittels, M. and Sherrill, F. A., Phys. Rev. 93, 1117 (1954).
81.EerNisse, E. P., J. Appl. Phys. 45, 167 (1974).
82.Presby, H. M. and Brown, W. L., Appl. Phys. Lett. 24, 511 (1974).
83.Arnold, G. W., Radiat. Eff. 65, 17 (1982).
84.Sato, S., Furuya, H., Inagaki, Y., Kozaka, T., and Sugisaki, M., J. Nucl. Sci. Technol. 24, 920 (1987).
85.Sato, S., Furuya, H., Asakura, K., Ohta, K., and Tamai, T., Nucl. Instrum. Methods in Phys. Res. B 1, 534 (1984).
86.Shelby, J. E., J. Appl. Phys. 51, 2561 (1980).
87.Primak, W. and Kampwirth, R., J. Appl. Phys. 39, 6010 (1968).
88.Norris, C. B. and EerNisse, E. P., J. Appl. Phys. 45, 3876 (1974).
89.Arnold, G. W., in Scientific Basis for Nuclear Waste Management VIII, edited by Jantzen, C. M., Stone, J. A., and Ewing, R. C. (Mater. Res. Soc. Symp. Proc. 44, Pittsburgh, PA, 1985), p. 617.
90.Hiraiwa, A., Usui, H., and Yagi, K., Appl. Phys. Lett. 54, 1106 (1989).
91.Antonini, M., Manara, A., and Buckley, S., Radiat. Eff. 65, 55 (1982).
92.Antonini, M., Manara, A., and Lensi, P., in Physics of SiO2 and its Interfaces, edited by Pantiledes, S. T. (Pergamon, New York, 1978), p. 316.
93.Devine, R. A. B. and Marchand, M., Appl. Phys. Lett. 63, 619 (1993).
94.Fukumi, K., Chayahara, A., Satou, M., Hayakawa, M., Hangyo, M., and Nakashima, S., Jpn. J. Appl. Phys. 29, 905 (1990).
95.Wright, A. C., J. Non-Cryst. Solids 179, 84 (1994).
96.Weeks, R. A., J. Appl. Phys. 27, 1376 (1956).
97.Weeks, R. A., Phys. Rev. 130, 570 (1963).
98.Griscom, D. L., Nucl. Instrum. Methods in Phys. Res. B 1, 481 (1984).
99.Feigl, F. J., Fowler, W. B., and Yip, K. L., Solid State Commun. 14, 225 (1974).
100.Yip, K. W. and Fowler, W. B., Phys. Rev. B 11, 2327 (1975).
101.Snyder, K. C. and Fowler, W. B., Phys. Rev. B 48, 13 238 (1993).
102.Weeks, R. A., Proc. VII Intl. Cong. on Glass, Brussels, Paper No. 41 (1965).
103.Tohmon, R., Mizuno, H., Ohki, Y., Sasagane, K., Nagasawa, K., and Hama, Y., Phys. Rev. B 39, 1337 (1989).
104.Imai, H., Arai, K., Hosono, H., Abe, Y., Arai, T., and Imagawa, H., Phys. Rev. B 44, 4812 (1991).
105.Griscom, D. L., J. Ceram. Soc. Jpn. 99, 923 (1991).
106.Amossov, A. V. and Rybaltovsky, A. O., J. Non-Cryst. Solids 75 (1994).
107.Griscom, D. L., in Proc. Thirty-Third Frequency Control Symposium (Electronics Industries Assn., Washington, DC, 1979), p. 109.
108.Hayes, W., Kane, M. J., Salimen, O., Wood, R. L., and Doherty, S. P., J. Phys. C: Solid State 17, 2943 (1984).
109.Tsai, T. E. and Griscom, D. L., Phys. Rev. Lett. 67, 2517 (1991).
110.Itoh, N., Shimizu-Iyayama, T., and Fujita, T., J. Non-Cryst. Solids 179, 194 (1994).
111.Edwards, A. H. and Fowler, W. B., Phys. Rev. B 26, 6649 (1982).
112.Pfeffer, R. L., in The Physics and Technology of Amorphous SiO2, edited by Devine, R. A. B. (Plenum Publishing, New York, 1988), p. 181.
113.Pfeffer, R. L., in The Physics and Chemistry of SiO2 and the Si-SiO2 Interface, edited by Helms, C. R. and Deal, B. E. (Plenum Press, New York, 1988), p. 169.
114.Friebele, E. J., Griscom, D. L., Stapelbroek, M., and Weeks, R. A., Phys. Rev. Lett. 42, 1346 (1979).
115.Stapelbroek, M., Griscom, D. L., Friebele, E. J., and Sigel, G. H., Jr., J. Non-Cryst. Solids 32, 313 (1979).
116.Griscom, D. L., J. Non-Cryst. Solids 68, 301 (1984).
117.Griscom, D. L., Sigel, G. H., Jr., and Ginther, R. J., J. Appl. Phys. 47, 960 (1976).
118.Friebele, E. J. and Griscom, D. L., in Defects in Glasses, edited by Galeener, F. L., Griscom, D. L., and Weber, M. J. (Mater. Res. Soc. Symp. Proc. 61, Pittsburgh, PA, 1986), p. 319.
119.Griscom, D. L., Friebele, E. J., Long, K. J., and Fleming, J. W., J. Appl. Phys. 54, 3743 (1983).
120.Arnold, G. W., Radiat. Eff. 98, 55 (1986).
121.Arnold, G. W., Nucl. Instrum. Methods in Phys. Res. B 1, 516 (1984).
122.Battaglin, G., Mea, G. Della, De Marchi, G., Mazzoldi, P., and Puglisi, O., J. Non-Cryst. Solids 50, 119 (1982).
123.Battaglin, G. Della, Mea, G., De Marchi, G., Mazzoldi, P., and Puglisi, O., Radiat. Eff. 64, 99 (1982).
124.DeNatale, J. F., Howitt, D. G., and Arnold, G. W., Radiat. Eff. 98, 63 (1986).
125.Schreurs, J. W. H., J. Chem. Phys. 47, 818 (1967).
126.Griscom, D. L., J. Non-Cryst. Solids 64, 229 (1984).
127.Cases, R. and Griscom, D. L., Nucl. Instrum. Methods in Phys. Res. B 1, 503 (1984).
128.Cases, R. and Griscom, D. L., in Proc. XVI Int'l Cong. Glass, Vol. 3, Glass Structure (1992), p. 53.
129.Griscom, D. L., J. Non-Cryst. Solids 6, 275 (1971).
130.Levy, P. W., Loman, J. M., and Kierstead, J. A., Nucl. Instrum. Methods in Phys. Res. B 1, 549 (1984).
131.Vannerberg, N-G., in Progress in Inorganic Chemistry 4 (1962), p. 125.
132.DeNatale, J. F. and Howitt, D. G., Am. Ceram. Soc. Bull. 61, 582 (1982).
133.DeNatale, J. F. and Howitt, D. G., Nucl. Instrum. Methods in Phys. Res. B 1, 489 (1984).
134.Heuer, J. P., Chan, H. W., Howitt, D. G., and DeNatale, J. F., in NuclearWaste Management II, edited by Clark, D. E., White, W. B., and Machiels, J. J. (Advances in Ceramics 20, The American Ceramic Society, Westerville, OH, 1986), p. 175.
135.Manara, A., Antonini, M., Camagni, P., and Gibson, P. N., Nucl. Instrum. Methods in Phys. Res. B 1, 475 (1984).
136.Adams, P. B. and Evans, D. L., Mater. Res. Sci. 12, 525 (1978).
137.Snoeks, E., Weber, T., Cacciato, A., and Polman, A., unpublished.
138.Snoeks, E., Ph.D. Thesis, Utrecht University (1995).
139.Arnold, G. W., Nucl. Instrum. Methods in Phys. Res. B 32, 504 (1988).
140.Klaumünzer, S., Radiat. Eff. 110, 78 (1989).
141.Benyagoub, A., Löffler, S., Rammansee, M., and Klaumünzer, S., Nucl. Instrum. Methods in Phys. Res. B 65, 228 (1992).
142.Griscom, D. L., in Experimental Techniques of Glass Science, edited by O., El-Bayoumi and Simmons, C. J. (The American Ceramic Society, Westerville, OH, 1993), p. 161.
143.Griscom, D. L., J. Chem. Phys. 55, 1113 (1971).
144.Marples, J. A. C., Nucl. Instrum. Methods in Phys. Res. B 32, 480 (1988).
145.Inagaki, Y., Furuya, H., Idemitsu, K., Banba, T., Matsumoto, S., and Muraoka, S., in Scientific Basis for Nuclear Waste Management XV, edited by Sombret, C. G. (Mater. Res. Soc. Symp. Proc. 257, Pittsburgh, PA, 1992), p. 199.
146.Banba, T., Matsumoto, S., Muraoka, S., Yamada, K., Saito, M., Ishikawa, H., and Sasaki, N., in Scientific Basis for Nuclear Waste Management XVIII, edited by Murakami, T. and Ewing, R. C. (Mater. Res. Soc. Symp. Proc. 353, Pittsburgh, PA, 1995), p. 1397.
147.Antonini, M., Camagni, P., Lanza, F., and Manara, A., in Scientific Basis for Nuclear Waste Management-2, edited by Northrup, C. J. M. Jr (Plenum Press, New York, 1980), p. 127.
148.Sato, S., Furuya, H., Kozaka, T., Inagaki, Y., and Tamai, T., J. Nucl. Mater. 152, 265 (1988).
149.Manara, A., Gibson, P. N., and Antonini, M., in Scientific Basis for Nuclear Waste Management-V, edited by Lutze, W. (Mater. Res. Soc. Symp. Proc. 11, North-Holland, New York, 1982), p. 349.
150.Stoneham, A. M., Nucl. Instrum. Methods in Phys. Res. B 91, 1 (1994).
151.Roberts, F. P., Jenks, G. H., and Bopp, C. D., Radiation Effects in Solidified High-LevelWastes–Part 1, Stored Energy, BNWL-1944 (Pacific Northwest National Laboratory, Richland, WA, 1976).
152.Hall, A. R., Dalton, J. T., Hudson, B., and Marples, J. A. C., in Management of Radioactive Wastes from the Nuclear Fuel Cycle, Vol. II, IAEA-SM-207 (International Atomic Energy Agency, Vienna, 1976), p. 3.
153.Malow, G., Marples, J. A. C., and Sombret, C., in Radioactive Waste Management and Disposal, edited by Simon, R. and Orlowski, S. (Harwood Academic Publishers, Chur, Switzerland, 1980), p. 341.
154., A.K., Luckscheiter, B., Lutze, W., Malow, G., and Schiewer, E., Am. Ceram. Soc. Bull. 55, 500 (1976).
155.DeNatale, J. F. and Howitt, D. G., Radiat. Eff. 91, 89 (1985).
156.Weber, W. J., Turcotte, R. P., Bunnell, L. R., Roberts, F. P., and Westsik, J. H., in Ceramics in Nuclear Waste Management, edited by Chikalla, T. D. and Mendel, J. E., CONF-790420 (National Technical Information Service, Springfield, VA, 1979), p. 294.
157.Sato, S., Asakura, K., and Furuya, H., Nucl. Chem. Waste Management 4, 147 (1983).
158.DeNatale, J. F. and Howitt, D. G., Am. Ceram. Soc. Bull. 66, 1393 (1987).
159.Heuer, J. P., Thesis, M. S., Department of Mechanical Engineering, University of California–Davis 1987.
160.Howitt, D. G., Chan, H. W., DeNatale, J. F., and Heuer, J. P., J. Am. Ceram. Soc. 74, 1145 (1991).
161.Tosten, M. H., TEM examination of irradiated waste glass, WSRCRP 89-584 (Westinghouse Savannah River Co., Aiken, SC, 1989).
162.Bibler, N. E., Tosten, M. H., and Beam, D. C., in High-Level Radioactive Waste Management, Vol. 2 (American Nuclear Society, La Grange Park, IL, 1990), p. 1103.
163.Laval, J. Y. and Westmacott, K. H., in Electron Microscopy and Analysis, 1979, edited by Mulvey, T., Conference Series, No. 52 (Institute of Physics, London, 1980), p. 295.
164.Inagaki, Y., Furuya, H., Ono, Y., Idemitsu, K., Banba, T., Matsumoto, S., and Muraoka, S., in Scientific Basis for Nuclear Waste Management XVI, edited by Interrante, C. G. and Pabalan, R. T. (Mater. Res. Soc. Symp. Proc. 294, Pittsburgh, PA, 1993), p. 191.
165.Matzke, Hj. and Toscano, E., Europ. Appl. Res. Rep. 7 (9), 1403 (1990).
166.Matzke, Hj. and Vernaz, E., J. Nucl. Mater. 201, 295 (1993).
167.Matzke, Hj. and van Geel, J., in Disposal of Weapons Plutonium, edited by Merz, E. R. and Walter, C. E. (Kluwer Academic Publishers The Netherlands, 1996), p. 93.
168.Bonniaud, R. A., Francillon, N. R. Jacquet, Laude, R. L., and Sombret, C. G., in Ceramics in Nuclear Waste Management, edited by Chikalla, T. D. and Mendel, J. E., CONF-790420 (National Technical Information Service, Springfield, VA, 1979), p. 57.
169.Routbort, J. L. and Matzke, Hj., Mater. Sci. and Eng. 58, 229 (1983).
170.Weber, W. J. and Matzke, Hj., Europ. Appl. Res. Rep. 7 (7), 1221 (1987).
171.Yamashita, M. and Matzke, Hj., in Modifications Induced by Irradiation in Glasses, edited by Mazzoldi, P. (Elsevier Science, Amsterdam, 1992), p. 53.
172.Ray, I. L. F. and Matzke, Hj., unpublished results.
173.Turcotte, R. P., Radioactive Waste Management 2, 169 (1981).
174.Dran, J. C., Langevin, Y., Maurette, M., Petit, J. C., and Vassent, B., in Scientific Basis for Nuclear Waste Management, edited by Topp, S. V. (Mater. Res. Soc. Symp. Proc. 6, North-Holland, New York, 1982), p. 651.
175.Primak, W., Nucl. Sci. Engr. 80, 689 (1982).
176.Cousens, D. R. and Myhra, S., J. Non-Cryst. Solids 54, 345 (1983).
177.Grover, J. R. and Chidley, B. E., Reactor Science and Technology (J. Nucl. Energy Parts A/B) 16, 405 (1962).
178.Grover, J.R., in Management of Radioactive Wastes from Fuel Reprocessing (Organisation for Economic Co-Operation and Development, Paris, 1973), p. 593.
179.Westsik, J. H. and Harvey, C. O., High-Temperature Leaching of a Simulated High-Level Waste Glass, PNL-3172 (Pacific Northwest Laboratory, Richland, WA, 1981).
180.Eyal, Y. and Fleischer, R. L., Geochimica et Cosmochimica Acta 49, 1155 (1985).
181.Olander, D. R. and Eyal, Y., Geochimica et Cosmochimca Acta 54, 1889 (1990).
182.Ellison, A. J. G. and Navrotsky, A., J. Am. Ceram. Soc. 75, 1430 (1992).
183.Ellison, A. J. G. and Hess, P. C., J. Non-Cryst. Solids 127, 247 (1991).
184.Calemezuk, R. and Bonjour, E., J. Non-Cryst. Solids 43, 427 (1981).
185.Navrotsky, A., Transaction ACA 27, 1 (1991).
186.Susman, S., Volin, K. J., Liebermann, R. C., Gwanmesia, G., and Wang, Y., Phys. Chem. Glasses 31, 144 (1990).
187.Hemley, R. J., Mao, K. K., Bell, P. M., and Mysen, B. O., Phys. Rev. Lett. 57, 747 (1986).
188.Stolen, R. H., Krause, J. T., and Kurkijan, C. R., Discuss. Faraday Soc. 50, 103 (1970).
189.Griscom, D. L., SPIE 541, 38 (1985).
190.Arnold, G. W. and Compton, W. D., Phys. Rev. 116, 802 (1959).
191.Pfeffer, R. L., J. Appl. Phys. 57, 5176 (1985).
192.Arnold, G. W. and Mazzoldi, P., in Ion Beam Modification of Insulators, edited by Mazzoldi, P. and Arnold, G. W. (Elsevier, Amsterdam, 1987), Chap. 5.
193.Mazzoldi, P. and Miotello, A., Radiat. Eff. 98, 205 (1986).
194.Miotello, A. and Mazzoldi, P., J. Phys. C: Solid State Phys. 15, 5615 (1982).
195.Miotello, A., Phys. Lett. 103A, 279 (1984).
196.Weber, W. J., Ewing, R. C., and Wang, L. M., J. Mater. Res. 9, 688 (1994).
197.James, P. F., J. Mater. Sci. 10, 1802 (1975).
198.Phase Separation in Glass, edited by Mazurin, O. V. and PoraiKoshits, E. A. (North-Holland, Amsterdam, 1984).
199.Taylor, P., Atomic Energy of Canada Limited Report, AECL-10173, August, 1980.
200.Haller, W., Blackburn, D. H., Wagstaff, F. E., and Charles, R. J., J. Am. Ceram. Soc. 53, 34 (1970).
201.Fudali, R. F., Dayar, M. D., Griscom, D. L., and Schreiber, H. D., Geochim. Cosmochim. Acta 51, 2749 (1987).
202.Chiang, Y-M. and Kingery, W. D., J. Am. Ceram. Soc. 66, C171 (1983).
203.Sreeram, A. N. and Hobbs, L. W., in Beam-Solid Interactions: Fundamentals and Applications, edited by Nastasi, M., Harriott, L. R., Herbots, N., and Averback, R. S. (Mater. Res. Soc. Symp. Proc. 279, Pittsburgh, PA, 1993), p. 559; A. N. Sreeram, Sc.D. Thesis, MIT (1995).
204.Spilman, D. B., Hench, L. L., and Clark, D. E., Nucl. Chem. Waste Management 6, 107 (1986).
205.Hobbs, L. W., Clinard, F. W. Jr, Zinkle, S. J., and Ewing, R. C., J. Nucl. Mater. 216, 291 (1994).
206.Yu, J., Sommer, W. F., and Bradbury, J. N., J. Nucl. Mater. 141–143, 65 (1986); J. Yu, W. F. Sommer, J. N. Bradbury, W. V. Green, and M. Victoria, J. Nucl. Mater. 227, 266 (1996).
207.Hobbs, L. W., in Quantitative Electron Microscopy, edited by Chapman, J. N. and Craven, A. J. (Scottish Universities Summer Schools in Physics Publ., Edinburgh, 1984), p. 399; Scanning Microscopy, Suppl. 4, 171 (1990).
208.Catlow, C. R. A., Diller, K. M., and Hobbs, L. W., Philos. Mag. 42, 123 (1980).
209.Hobbs, L. W., J. Phys. 37 (C7), 3 (1976).
210.Computer Simulation of Radiation Effects in Solids, edited by T., Diaz de la Rubia, G.H., Gilmer, and M-J., Caturla (North Holland, Amsterdam, 1995).
211.Adams, J. B., Rockett, A., Kieffer, J., Xu, W., Nomura, M., Kiliam, K. A., Richards, D. F., and Ramprasad, R., J. Nucl. Mater. 216, 265 (1994).
212.Mattila, T., Nieminen, R. M., and Dzugutov, M., Nucl. Instrum. Methods in Phys. Res. B 102, 119 (1995).
213.Doan, N. V., Philos. Mag. A49, 683 (1984).
214.Valle, R. G. Della and Andersen, H. C., J. Chem. Phys. 97, 2682 (1992).
215.Cormier, G., Peres, T., and Capobianco, J. A., J. Non-Cryst. Solids 195, 125, (1996).
216.Vessal, B., Wright, A. C., and Hannon, A. C., J. Non-Cryst. Solids 196, 233 (1996).
217.Cormack, A. N. and Cao, Y., Mol. Eng. (1996), in press.
218.Delaye, J. M. and Ghaleb, D., J. Non-Cryst. Solids 195, 239 (1996).
219.Delaye, J. M. and Ghaleb, D., Mater. Sci. Eng. B37, 232 (1996).
220.Delaye, J. M., presented at this panel meeting (unpublished).
221.Delaye, J. M. and Ghaleb, D., J. Nucl. Mater. (in press).
222.Delaye, J. M. and Ghaleb, D., in Proc. of the Third International Conference on Computer Simulations of Radiation Effects in Solids, University of Surrey, Guildford, UK, July 22–26, 1996.
223.Wicks, J. D. and McGreevy, R. L, J. Non-Cryst. Solids 192/193, 23 (1995).
224.Wicks, J. D., Börjesson, L., Bushnell-Wye, G., Howells, W. S., and McGreevy, R. L., Phys. Rev. Lett. 74, 726 (1995).
225.Park, J-G. and Cormack, A. N., Philos. Mag. B 73, 21 (1996).
226.Brailsford, A. D. and Bullough, R., J. Nucl. Mater. 44, 121 (1972).
227.Jain, U. and Lidiard, A. B., Philos. Mag. 35, 245 (1977).
228.Yu, N., Nastasi, M., Levine, T. E., Tesmer, J. R., Hollander, M. G., Evans, C. R., and Maggiore, C. J., Nucl. Instrum. Methods in Phys. Res. B 99, 566 (1995).
229.Allen, C. W., Funk, L. L., Ryan, E. A., and Taylor, A., Nucl. Instrum. Methods in Phys. Res. B 40/41, 553 (1989).

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